Book of Abstracts


The material in this book has been supplied by the autors and has not been corrected by the Programme Committee of the Symposium. The views expressed remain the responsibility of the named authors. In particular, neither the Programme Committee nor any organization or body sponsoring this meeting can be held responsible for any material reproduced in this book.


SESSION I:
RADIATION PROTECTION AT WORKPLACE


OP1

THE CENTRAL REGISTRIES OF OCCUPATIONAL AND MEDICAL EXPOSURE IN THE CZECH REPUBLIC

K. Petrova, Z. Prouza

National Institute of Public Health, Radiation Hygiene Centre, Czech Republic

The authors present and discuss in their paper reasons for the creation of central registries of exposure to ionizing radiation and inform on recent status in this field world-wide and in the Czech Republic. The creation of the Central Registry of Occupational Radiation Exposure (CR ORE) has been prepared in the Czech Republic since 1993 , when the detailed analyse of status in this area in our country was done. The actions leading to the creation of the CR ORE were opened in 1994 under the financial participation of the Ministry of Industry and Trade. Following steps have been already done: the choose of the company for software covering of the system, the enter into the co-operation with the Central Service of Personal Dosimetry and dosimetric services operating in NPP and uranium industry, the effort on a methodology unification of a dosimetric evaluation of the occupational exposure. The contact with the International System on Occupational Exposure was also opened up in 1994 and the created national system of ORE registration is built in the harmony with the recommendations and demands of this international system. The paper gives more detailed information on the structure of creating program and discuss some actual arising problems.

The preparation of the Central Registry of Medical Radiation Exposure ( CR MRE) in the CR is recently in the stage of analyse of present status and approaches to the solution of this problem both world-wide and in the Czech Republic. New approach to the evaluation of medical exposures that can be recently observe in the world is taken in apart in a preparation of CR MRE in the CR. The attention is paid to the determination of the age and sex dose distributions for individual examinations. The authors show conclusions of UNSCEAR Report 1993 concerning to observation of medical exposures and discuss some specific problems conducting with the evaluation of radiation burden arising from medical exposures. The co-operation with some medical utilities , Institute of Health Information Systems of Ministry of Health and General Health Insurance Company was done to obtain necessary data on medical exposures in CR. The methodology of data collection and special database system for input and transfer of data is recently created. This system allows to distribute data according to demanded parameters. Presented are some partial results following from obtained data as yet.



OP2

RADIATION PROTECTION ASPECTS FOR A 40 MEV CYCLOTRON PLANT

P. Ragni, R. Horn-Orni

Istituto di Chimica Nucleare del C.N.R., Area della Ricerca Monterotondo Scato (RM), Italia
Ufficio di Sicurezza e Prevenzione del C.N.R., Via di Pietralata 190, Roma, Italia

It is foreseen the installation of a 40 MeV Scanditronix cyclotron with a PET facility in the new C.N.R. Research Area at Tor Vergata, about 20 km far from Rome. It will be the first medium size cyclotron for chemical and medical research in Italy and in the area of Mediterranean Countries and it is foreseen the start of research activities open to international cooperations and the production of PET and SPECT short-live radioisotope for medical purposes, also in order to supply some hospitals needs.

In the present work is reported the final building project and are briefly stressed the studies carried out to assure radiation protection requirements for the dangerous areas (shielding protections, duct holes, doors), also taking in account the new law prescriptions that are going to be approved.

Then are reported the main radiation protection criteria and procedures for PET and SPECT radioisotopes production, for liquid waste disposal and for airborne radioactivity.



OP3

DOSE MEASUREMENTS AND LET-DETERMINATION IN SPACE STATION MIR DURING THE RUSSIAN LONG TERM FLIGHT RLF

N. Vana, W. Schöner, M. Fugger, Y. Akatov *

Atominstitute of the Austrian Universities, Schüttelstrasse 115, A-1020 Vienna, Austria
* Institute for Biomedical Problems (IMBP), Choroshovskoje shosse 76 A, 123 007 Moscow, Russia

For determination of the absorbed dose and the dose equivalent in complex mixed radiation fields, new methods were developed in the frame of the Austrian-Soviet space mission AUSTROMIR in October 1991. The method utilizes the changes of peak height ratios in thermoluminescence glowcurves. Peak height ratios depend on the linear energy transfer (LET) of absorbed radiation. This effect was calibrated in different radiation fields (alpha-, beta-, gamma-, neutron fields and heavy charged particle beams). The method was approached for dose measurements during several space programmes (DOSIMIR, BION-10, PHOTON-8).

During the Russian long term flight RLF six dosemeter packets were exposed in three different periods. Two places with different shielding (the working area and the cabin of the board engineer) were chosen for exposition of the dosemeters during each period in order to measure the variation of absorbed dose as well as the variation of average LET of absorbed radiation within the habitable part of space station MIR. These results will be compared with the results during two former periods of measurements on space station MIR (AUSTROMIR/DOSIMIR) and results obtained inside of biosatellite BION-10 and the space shuttle mission STS-60.

Work supported by the Austrian Society for Aerospace Medicine, ASM



OP4

DETERMINATION OF PATIENT SURFACE DOSE FROM COMPUTED TOMOGRAPHY EXAMINATIONS OF THE BODY

B. Vekic 1, S. Kovacevic 1, M. Ranogajec-Komor 1, N. Duvnjak 2, P. Marusic 2, P. Anic 3, P. Dolencic 3

1 Rudzer Boskovic Institute, Zagreb, Croatia
2 New Hospital, Zagreb, Croatia
3 University Hospital "Merkur", Zagreb, Croatia

Computed tomography (CT) has become a major source of the population exposure to diagnostic X-rays, and the knowledge of the doses delivered by the CT equipment has become very important. Considerable efforts should be made to keep these doses to a reasonable minimum, without sacrificing the image quality. The conditions of exposure in CT are quite different from those in conventional X-ray imaging. This has required the development of specific techniques for assessing patient dose from CT. The aims of this work were to determine the doses delivered to various organs of patients undergoing computed tomography of abdomen and thorax as measured on the surface of the body and to estimate the risk to the patients.

Dosimetric measurements were performed at two different CT scanners (Siemens SOMATOM DR-H, ver. HC-l and Shimadzu SCT-4500TE). The doses absorbed by different organs (gonads, chest, thyroid and eye lens) and by the examined part of the body of 44 patients of various sex and age were measured with TLD-700.

The doses absorbed by different organs during the diagnostic CT examination of the body depended on the technical parameters, such as the number of scans, mAs, the thickness of scans, scanning times, tube voltage and other characteristics, some of which depended on the type and severity of illness, Clinical parameters, such as patient size and composition and patient cooperation with regard to control and motion, also influence the dose and the image quality. The highest dose measured in this study (89.19 mGy) was delivered to kidney during CT examination of this organ.



OP5

METHODS TO IMPROVE RADIOPROTECTION FOR BAITA-PLAI (ROMANIA) URANIUM MINERS

S. Ramboiu

Medical Center and Health Services and Management, Cluj-Napoca, Romania

Workers in uranium nine are subjected to the risk of internal contamination by Radon-222 and Radon-222 short-lived progeny inhalation.

The paper presents some methods to improve radioprotection of workers in "Avram Iancu" uranium mine, on the basis of simultaneous measurements of Radon-222 and its progeny concentrations in the underground air.

Kuznetz's and Rock's methods were used to measure Radon-222 and Radon-222 short-lived progeny concentrations in air, respectively.

Internal contamination of workers in "Avram Iancu" uranium mine is indirectly evaluated by multiplying the weakly measured Radon-222 concentrations in air by a constant value of the equilibrium factor between Radon-222 and progeny, of 30%.

As a consequence of an insufficient flow rate of air, the concomitant determinations of Radon-222 and its progeny reveal that the equilibrium factors ranged between 20% and 80% . So, the utilisation of the equilibrium factor of 30 % had to an under evaluation of internal doses.

The method proposed in the aim to improve the estimation of the individual internal doses consist in a monthly determinations of equilibrium factors in all working places.

The methods to improve the underground ventilations are also presented.



PP1

MEASUREMENT OF C-14 INSIDE THE KRSKO NUCLEAR POWER PLANT

B. Vokal, J. Burger, T. Mohar, M. Franko and I. Kobal

Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia

One of the most important radionuclides released to the environment from nuclear power plants is carbon-14. It is produced in light water reactors by neutron activation of oxides and by the reaction of impurities, such as nitrogen, in the fuel, moderator and coolant. C-14 is mainly released to the environment in stack gas. However, uncontrolled releases of C-14 can also occur during maintenance and various repair work inside the nuclear power plant.

For this reason it was the objective of this work to monitor C-14 inside the Krsko Nuclear Power Plant. Air was continuously taken at several locations inside the plant by a CO2/CH4 sampler for two week periods. CO2 was absorbed in a potassium hydroxide trap and then the hydrocarbons were converted into CO2 by a Pd catalyst kept at 600 C and removed in a second potassium hydroxide trap. Sample activities were measured by liquid scintillation counting (LSC) after precipitation of carbonate with BaCl2 in the form of BaCO3.

Variations in radioactive CO2 and hydrocarbon concentrations in air at various locations in the plant will be reported.



PP2

CITOGENETIC MONITORING OF MEDICAL PERSONNEL WORKING IN A DEPARTMENT OF UROLOGY

K. Sentija, V. Kasuba

Institute for Medical Research and Occupational Health, Ksaverska cesta 2, 41000 Zagreb, Croatia

Cytogenetic monitoring for long term exposure to low-level ionizing radiation was evaluated. Peripheral blood samples from 21 subjects working in a department of urology were collected and cultivated for standard chromosome aberration method. All chromosome-type aberrations i.e. isochromatid breaks, dicentrics and rearrangements were considered and compared to control. The medical personnel consisted of physicians, nurses and technicians professionally exposed to low-level ionizing radiation for 17.3 years in average. Among them, a subgroup of 12 subjects performed urological diagnostic and therapeutical ultrasound procedures for the last 7.1 years. A higher percentage of total aberrations, and a significant increase of chromosome breaks, rings, dicentric chromosomes and acentric fragments was observed in the exposed group compared to control. Comparing the ultrasound subgroup with the rest of the exposed personnel, a significant increase of chromatid breaks and rings was noted. Correlating duration of exposure to ultrasound and chromosome aberrations, a positive correlation for chromosome breaks, acentrics and dicentrics was found. Apart from confirming ionizing radiation as a radiomimetic agent, our results point out ultrasound as a potentially additional contributing factor in chromosome damage.


PP3

HEALTH SURVEILLANCE OF MEDICAL PERSONNEL OCCUPATIONALLY EXPOSED TO IONIZING RADIATION SOURCES: BIOMONITORING AND DOSIMETRY

V. Brumen, I. Prlic, Z. Radalj, D. Horvat and H. Cerovac

Institute for Medical Research and Occupational Health Zagreb, 2 Ksaverska street, POB 291, Zagreb, Croatia

The aim of this work is to present the complete results of periodical health surveillance of medical personnel occupationally exposed to ionizing radiation sources, conducted according to established law regulations in Croatia. The report comprises a total of 21 examinees (11 female, 10 male), mean age 43,19 +- 9,85 years, originating from different professional groups and working in a radiation zone l4,7 +- 8,27 years on the average. Within the framework of this study, the results of their biomonitoring, including haematological parameters (whole blood count), ophthalmological findings (fundus oculi), cytogenetic test (conventional structural chromosomal aberration analysis) and peripheral blood flow survey (capillaroscopy and dermothermometry) will be presented. Filmdosimetric data for the referred period will also be reported.


PP4

IOD-131 AIR CONTAMINATION IN SOME NUCLEAR MEDICINE CENTERS

M. Bayer *, N. Muntean *, T. Fiat **, L.Daraban **

* Medical Center and Health Services and Management, Cluj, Romania
** Babes Bolyai University, Faculty of Physics, Cluj-Napoca, Romania

The paper presents the Iod-131 contamination of the atmosphere within some nuclear medicine centers unit in Cluj-Napoca and Baia Mare towns. The air samples were collected in different workrooms e.g. laboratories for the first dilution and administrative and measuring offices.

The used working method was based on filtering a definite air volume through an active coal filter who is impregnated with AgNO3 solution. The I-131 retained was measured with the well-type NaI(Tl) crystal scintillation counter connected to an impulse meter with an efficiency to 20 % to 40 % the efficiency of filtration was 90 % and the minimum detectable activity was 1.11 Bq/m.c.

In 1991 the filtering cartridge was replaced by a SLF-2I-50 special filter for radio iodine.

The registered values ranging between 1.11 Bq/m.c. and 29.63 Bq/m.c. are situated below the admissible levels of the occupational exposure norms.

Accordingly, the studied nuclear medicine centers do present safe work conditions.



PP5

RADIATION PROTECTION IN CHEST RADIOGRAPHY IN CHILDREN UNDER ONE YEAR

C. Fulea, S. Ramboiu

Medical Center and Health Services and Management, Cluj-Napoca, Romania

The protection of reproductive organs in children during the pelvis radiography doses exert a direct effect in reducing the possible associated genetic risk. The heavy exposure of children undergoing pelvis X-ray examination require a practical method for diminishing the irradiation at the level off the gonad area because at least 1% of the cases with ship dysplasia cannot be clinically diagnosed within the first months of life.

Our paper presents the design a hip mask for children (0-1 years) gonad protection during the pelvis radiography.

The doses absorbed by the radiosensitive organs were evaluated by the Monte Carlo calculation technique on the bases of the measurements effectuated by LIF thermoluminescent dosimeters in a group of 60 children.

Out of the total number of the basin radiography 86.4 % has been yearly applied in children within the first year of life to detect the hip congenital dysplasia.



SESSION II:
NATURAL RADIOACTIVITY


OP6

RADON RISK CLASSIFICATION OF FOUNDATION SOILS - SOME REMARKS

M. Neznal, M. Neznal, J. Smarda

RADON v.o.s. corporation, Za koncem 1380, 289 22 Lysa nad Labem, Czech Republic

The uniform method for radon risk classification of foundation soils used in the Czech Republic is based on the soil-gas radon concentration measurement and on the determination of soil permeability. The first proposal was given in 1990. Three categories of risk were defined - low, medium and high risk of radon infiltration from the ground. A four years experience has resulted in some modifications of the origin classification method. The modifications were recommended in 1994. RADON v.o.s. corporation participated in solving several research projects that concerned further improvement of the method.

As for practical applicability of radon survey results, it seems useful to define a single parameter (radon availability) for characterizing the radon potential of soils. Different ways how to define this parameter will be presented and discussed.



OP7

SOME PROBLEMS ON RADON REFERENCE MEASUREMENT SYSTEM AND RADON INDOOR-OUTDOOR MONITORING

X. Myteberi 1, P. DeFelice 2

1 Institute Of Nuclear Physics, Tirana, Albania
2 National Institute Of Radiation Metrology, ENEA,CRE Casaccia, Rome, Italy

One important requirement for accurate monitoring of Radon in working environment and/or dwellings is to ensure the necessary reliability and traceability.

A Rn-222 Reference Measurement System recently developed in the same way at ENEA and INP is presented. It is based on a Radon transfer counting system calibrated by some Ra-226 standard liquid solution traceable to the international system. Reference counting instruments are cylindrical electrostatic cells equipped with Si detectors. It is used for the detection of the electrostatically collected Po-118 and Po-214 ions produced in the decay of Rn-222. The activity of Rn-222 gas in a spherical glass bulb can be measured by the Reference System, by a particular procedure that does not requires the calculation of any volume ratio of any assumption of total radon removal from the liquid Ra-226 solution. The overall uncertainty estimated for the calibration of Rn-222 sources is about 1% at the 68% confidence level.

The measurement systems and operational procedures adopted for Radon metrology are described. The paper also reports the participation of ENEA in the 2nd EUROMET intercomparison of the Rn-222 measurement systems of a number of European labs, and the efforts performed to stabilize the traceability of INP to ENEA.

The possibilities of calibration for some passive detectors by the above system are discussed.

References:

  1. J.M.Hutchinso, App.Radiat. Isot. vol 43,1/2,175,(1992),
  2. R.Falk, J.Res.Nat.Inst.Stand.Tech. 95,115(1992),
  3. R.F.Holub, J.Res.Nat.Inst.Stand.Tech. 95, 121(1992),
  4. R.Colle, J.Res.Nat.Inst.Stand.Tech. 95, 155(1992),
  5. P.DeFelice, Xh.Myteberi, Paper accepted to be presented at ICRM '95 Paris May (1995),
  6. Xh. Myteberi,P.Skende, Proceedings of ENVIRONMENT '94, Conference organized by Universities of Tirana,Academy of Sciences and Ministry of Health of Albania (1994).



OP8

ENVIRONMENTAL RADIOACTIVE CONTAMINATION CAUSED BY THE URANIUM EXTRACTION INDUSTRY AND PROBLEMS OF SITE REMEDIATION IN THE EAST EUROPEAN COUNTRIES

J. Fietz

Research Center Rossendorf (FZR), Germany

Uranium ore mining and processing leads to the release of natural radionuclides into the biosphere and so enhances their natural concentrations in the near-site environment. Radionuclides of the uranium progeny are concentrated mainly in the processing residues (tailings), but also in lean ore and rock heap dumps, in deep and in surface waters and in the atmosphere. The additional exposure of the residents to these pollutants has to be restricted by an ecologically orientated production as well as by thorough remediation after closing-down of the site.

According to the classification of the ICRP, site contamination by natural radionuclides represents a "pre-existing" situation, that can only be influenced by intervention. The dose limits do not apply in this case and are replaced by recommended levels, which depend on the specific situation. Concerning the remediation of uranium production sites, an effective dose equivalent of 1 mSv/a above the natural level has been introduced as a primary criterion in most countries. From this criterion secondary quantities are derived for activity concentrations in different environmental media and for radon exhalation rates.

In the former Eastern Bloc countries about 700 000 t uranium were produced from 1945 - 1993. This production mainly followed military-industrial demands, ecological aspects were largely subordinated to it. Therefore, site remediation for many of the recently closed-down installations will prove a very expensive process both under technical and financial aspects.

Following a review of uranium production in Eastern Europe and in the Asian CIS-countries, the radiological situation for selected sites is analyzed, and basic demands for remediation programs are discussed.



OP9

A NATIONAL SURVEY OF INDOOR RADON CONCENTRATIONS IN DWELLINGS IN SLOVENIA

R. Ilic, M. Krizman, J. Skvarc, Z. Jeran

Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia

In the period December 1993 - February 1994 long term concentrations of indoor radon were measured in 892 randomly selected dwellings in Slovenia with a passive radon dosemeter, utilizing CR-39 etched track detector. The latent track images were transformed to visible tracks by the electrochemical etching technique; the numbers of tracks were evaluated by the TRACOS automatic image analysis system.

The measured data cover the whole territory of Slovenia quite uniformly. Compared to the total number of buildings (463.000 houses), approximately every 500th house was examined. Results were statistically evaluated and modified for seasonal corrections. Maps of indoor radon concentrations in Slovenia were constructed in different formats, including those of grid squares (5 km x 5 km, 10 km x 10 km) and one with concentration isolines. Average annual concentrations in all communities were also determined and are presented on a separate map. The approximate median annual average concentration was found to be 54 Bq/m3, the arithmetic mean concentration was 87 Bq/m3, and the geometric mean 59 Bq/m3.

The main conclusions derived from this work are the following:

- The highest levels of indoor radon were found in the southern part of Slovenia (Karst, Lower and Inner Carniola); the group average for a single community vary from 160 - 280 Bq/m3,
- Higher concentrations were found in rural regions, especially in old detached houses; concentrations in larger towns are essentially lower,
- The radon maps reflect the findings of the map of natural radioactivity of the country: regions of the highest uranium/radium content in soil mostly coincide with high radon areas.

Based on the methodology of dose assessment following ICRP 50 recommendations, the average annual effective dose equivalent due to inhalation of indoor radon was estimated. The value obtained of 2 mSv per year is nearly the same as found in neighbouring countries.

The intervention level for indoor radon, based on a statistical analysis of the results of indoor radon concentrations and the criterion for high radon areas according to ICRP 65 recommendations, was derived. Remedial action should be taken when radon levels exceed the recommended action level of 400 Bq/m3; for new dwellings radon in future should not be greater than 200 Bq/m3.

As a result of this work Slovenia may be categorized in the group of countries with a well defined status of natural radioactivity: there will no longer be a blank area on the radiological map of Europe.



OP10

THE 222RN TRANSFER MEASUREMENT SYSTEM DEVELOPED AT ENEA

P. DeFelice, Xh. Myteberi *

Instituto Nazionale di Metrologia delle Radiazioni Ionizzati, ENEA Dip. Ambiente, Centro Ricerche CASSACIA, Roma, Italy
* Institute of Nuclear Physics, Tirana, Albania

A 222Rn Transfer Measurement System was recently developed at ENEA, the Italian Primary Standard Institute for Ionising Radiation Quantities. This system is based on a NaI(Tl) well type detector calibrated by a set of standard radon gas sources in glass bulbs traceable to the ENEA 222Rn Reference Measurement System. The Transfer Measurement System has been characterized in terms of several additional parameters such as the operating range, the linearity and reproducibility of the system response, the short-term and long-term stability. The Transfer Measurement System is now used, at ENEA, for the non-destructively calibration of 222Rn gas sources in glass bulbs, with a combined uncertainty of about 1% (1 sigma).These sources are then used for production of standard radon atmospheres in the two ENEA radon chambers. The paper describes the Transfer Measurement System, the procedure adopted for its calibration and the results of other characterization tests. The paper also reports the participation of ENEA in a EUROMET intercomparison of the 222Rn measurement systems of a number of European laboratories carried out in 1994. A short outline is finally given of the other calibration facilities developed at ENEA for radon metrology.


OP11

FORMATION WATERS FROM OIL AND NATURAL GAS PRODUCTION -POTENTIAL POLLUTING SOURCE BY RADIUM 226

T. Peic, G. Dinca, I. C. Dutu, R. Peic, G. N. Sandor

Research and Design Institute for Rare and Radioactive Metals-Research Laboratory for Radiation Protection, Working Conditions and Ecology- Petru Groza Town, Romania

The polluting potential with radium 226 of formation waters from oil and natural gas fields was reported in 1983 by the Research Laboratory for Radiological protection from Petru Groza-Bihor. From 574 samples of formation waters arising from wells from different parts of country, 318 (55%) had a radium 226 content exceeding the MPC for drinking water, ranging from 0.16 Bq/L to 60.74 Bq/L. The fact that these waters are not injected in all situation, being discharged into watercourses or on agricultural lands, imposed further investigations. So, 40 oil treating stations and 8 natural gas ones were investigated. The results confirmed the pollution by radium of certain watercourses as well as of soil and vegetation. The radioactive crusts from tubing or other devices can contribute to the internal contamination of the workers.

The presence of over 15.000 wells and of over 50.000 hectares polluted by oil products underlines the necessity of approaching the problems related to polluting formation waters due to their high radium 226 content.



OP12

VARIATION AND ORIGIN OF ENHANCED RADON EXHALATION IN NORTH-EAST HUNGARY

G. Marx, E. Toth

Dept. of Atomic Physics, Eötv&oul;s University, Budapest, Hungary Lauder School, Budapest, Hungary

In 1992 an enhanced radon exhalation was discovered in the bedrooms of the village of Mtraderecske, reaching several thousand Bq/m3 in some living houses in yearly average. The mean radon activity concentration of the village is above 200 Bq/m3 in yearly average. The phenomenon is surprising because the rock is not especially rich in uranium. The radon exhalation is highly variable in time (year by year) and in space (within a few meters). The interest of the population made the survey practically in each house necessary in four seasons. The people have been informed and positive examples of radon migration have been realized. The origin of the radon has complex geophysical-geochemical reasons, that was studied by observing changes in time (in correlation with seismic activity and precipitation), by measuring radon in soil, rock, and well water. In this way a model for the origin of radon can be built up. The survey has been made able by the responsible unselfish cooperation of the teachers of the Lauder School and the school in Matraderecske, together with their students. it helped to increase the level of nuclear literacy among people. The survey has been supported by the OMFB and by the OTKA-T7603 project for buying instruments and detectors.


OP13

LOCAL DEPOSITION PATTERNS OF INHALED RADON PROGENY IN HUMAN BRONCHIAL AIRWAYS

T. Heistracher 1, W. Hofmann 1 and I. Balashazy 1,2

1 Institute of Physics and Biophysics, University of Salzburg, Austria
2 KFKI Atomic Energy Research Institute, Budapest, Hungary

The local distribution of radon decay products deposited within bronchial bifurcations, particularly the formation of hot spots, may be more relevant for the determination of cellular doses in bronchial tissue than the commonly computed deposition efficiency, which is conceptually equivalent to the assumption of a uniform nuclide distribution.

Particle deposition patterns within three-dimensional models of asymmetric bronchial airway bifurcations are simulated by a numerical fluid dynamics and particle trajectory model: (I) Airflow is computed by solving the Navier-Stokes equations with a finite volume method, (ii) trajectories of particles entrained in the airstream are simulated by Monte Carlo techniques, and, (iii) particle deposition patterns are determined by the intersection of the particle trajectories with the surrounding surfaces.

Inspiratory deposition patterns of 1 nm (unattached fraction) and 0.2 um (attached fraction) particles illustrate the formation of enhanced deposition sites at the carinal ridge, which is consistent with the action of strong local secondary flows. Such highly localized accumulations of radon decay products may produce high local cellular doses, which may significantly exceed dose estimates based on uniform nuclide distributions.



OP14

CELLULAR DOSIMETRY FOR RADON PROGENY ALPHA PARTICLES IN BRONCHIAL TISSUE

A. Mohamed 1, W. Hofmann 1 and I. Balashazy 1,2

1 Institute of Physics and Biophysics, University of Salzburg, Austria
2 KFKI Atomic Energy Research Institute, Budapest, Hungary

Inhaled radon progeny are deposited in different regions of the human bronchial tree as functions of particle size and flow rate. This initial deposition pattern is subsequently modified by radioactive decay, mucociliary clearance and transport through epithelial tissue into blood. Thus, sensitive bronchial basal and secretory cells are irradiated by two different alpha particle sources: (I) radon progeny in the sol and/or gel phase of the mucus layer, and (ii) radon progeny within the bronchial epithelium.

An analytical method has been used to compute the local energy deposition of Po-218 and Po-214 alpha particles in 1 m spheres located at different depths in bronchial epithelium. In order to reach the target, alpha particles travel either through tissue alone ( near wall" dose) or through air and tissue ( far wall" dose). While the depth-dose distributions for nuclides uniformly distributed within the epithelium are practically constant with depth, they decrease in an almost linear fashion with increasing depth for nuclides on the airway surface.

Histological studies have shown that the locations and relative frequencies of basal and secretory cell nuclei vary within a given bronchial airway generation and among different airway generations. Thus, different assumptions about cell-specific depths and their frequency distributions appreciably affect the related dose estimates.



OP15

LUNG CANCER RISK AMONG CZECH MINERS EXPOSED TO RADON

E. Kunz, L. Tomasek 1, V. Placek 1, T. Müller 2

1 National Institute of Public Health, Prague, Czech Republic
2 Institute of Occupational Hygiene in Uranium Industry, Kamenna, Czech Republic

Long term exposure to radon and its progeny is one of the most important health problems. Epidemiological studies have demonstrated that exposure of miners to radon in a mine atmosphere can cause lung cancer.

The presentation issues from data of the oldest Czechoslovak cohort study (N=4320), which belongs among the largest ones with the longest follow-up. By the end of 1990, a total of 700 lung cancers were observed. Individual exposures have been revised, particularly the recent working history of the miners.

The most recent analysis has shown that (similarly as in other cohorts of radon exposed miners) the excess relative risk of lung cancer per unit exposure is modified by time since exposure and exposure rate.

In addition in revising the data it has been found that the exposure revision had a great impact on the risk coefficient. This is also the main reason why the ERR/WLM coefficients reported during 1993-4 for this study were different. Observed findings are being verified from the point of view of histological types, which is available for about 67% of cases.



OP16

THE ASSESSMENT OF EXPOSURE TO RADON IN ROMANIAN NON-URANIUM MINES

G. N. Sandor, G. Dinca, T. Peic

Research and Design Institute for Rare and Radioactive Metals-Research Laboratory for Radiation Protection, Working Conditions and Ecology- Petru Groza Town, Romania

Between 1970-1993 were investigated 285 mining and exploration non-uranium units, at 114(40%)being exceeded the maximum permissible equilibrium equivalent concentration(MPC)of radon 222 for public (111Bq/m3) and at 15 (5,3%) the MPC for occupational exposure (1110Bq/m3), so being necessary the recommendation of limiting measures.

The causes of appearance and accumulation of radon have been clarified,the main source being the presence of natural radioactive elements in barren rocks and minerals and the cause of accumulation the inefficiency of ventilation.

The rock, mineral and water samples were analysed for their natural uranium and thorium and radium 226 content. On a PC were worked out the data regarding 2327 mineral samples, 5924 barren rock, 475 water ones, 3898 gamma dose rate measurements, and radon and radon daughters measurements from 3023 underground workplaces.

The mean individual annual effective doses for each type of useful mineral were assessed, these ranging from 0,77 mSv/year (salt mines) to 60,21 mSv/year (barytine mines).



OP17

ASSESSMENT OF RADON-DAUGHTER DEPOSITION IN THE RESPIRATORY TRACT

S. Oberstedt, H. Vanmarcke

Studiecentrum voor Kernenergie SCK.CEN, Boeretang 200, B - 2400 Mol, Belgium

Since some decades it is known, that most of the radiation dose to the lung is due to the inhalation of the short-lived decay products of 222Rn. Their deposition in the respiratory tract strongly depends on the attachment rate to aerosol-particles present in the indoor air and their plate-out rate to the surfaces. Instead of measuring the activity size distribution of the airborne decay products, knowledge on the respiratory tract retention has been incorporated in the design of a measurement system, called bronchial dosemeter, to assess the lung dose directly. The simulation of the deposition characteristics of the short-lived radon daughters in the nasal cavity and the bronchial tree is based on the comparison of the model of the respiratory tract with results from screen penetration theory. A bronchial dosemeter consisting of three sampling heads has been built and calibrated. Additionally, an outline of future activities will be given.


PP6

PRELIMINARY STUDY ON THE RATE OF BRONCHO-PULMONARY CANCER IN A ROMANIAN DEPARTMENT (BIHOR) FOR THE ESTIMATION OF RADON RISK EXPOSURE

T.Vaida 1, V.Pacurar 1, Fl.Maghiar 1, C.Cosma 2, D.Ristoiu 2, S. Ramboiu 2, A.Poffijn 3

1 Faculty of Medicine and Oncologic Centre Oradea, Romania
2 Faculty of Physics and Hygienic and Health Institute, Cluj-Napoca, Romania
3 Radon Research Group, University of Gent, Belgium

The best estimation of risk to which everyone is exposed from natural radon in buildings is now obtained by extrapolation from observation of men exposed to radon in mines. In the last years there are also some epidemiological studies which try to find out a direct connection between the lung cancer risk and the indoor radon concentration in buildings.

Our study follows the estimation of the rate of the primary broncho-pulmonary cancer in a period of two years (1993-1994) at the population in the Bihor district exposed probably at the increasing concentration of radon, heaving age between 15-80 years.

In these two years there are founded 471 cases of primary broncho-pulmonary cancer: 398 men (84.4%) and 73 women (15.6%). In 1993 were diagnosticated 234 new cases (190 men and 44 women) and in 1994 were founded 237 cases (208 men and 29 women).

For the epidemiological study were selected those ill persons who had the age between 40-75 years, in the moment of study's and those who leaved or leave more than 25 years in the Bihor district.



PP7

RADON EXPOSURES IN CAVES IN HUNGARY

I. Csige 1, I. Hunyadi 1, G. Geczy 2, J. Hakl 1 1 Institute of Nuclear Research of the Hungarian Academy of Sciences, H-4001 Debrecen, POB 51, Hungary
2 Eötvös Lordnt Univ. Dept. of Phys. Geog. H- 1 083 Budapest, Ludovika tdr 2, Hungary

We have estimated radon exposures from inhaled radon and its decay products (according to the proposals of the ICRP 65) for participants in speleotherapy in different Hungarian karstic caves. We have found, that about 5-10% of patients receive more than 5 mSv of effective dose equivalent during their cures, which value is a suggested annual limit of exposure of general population from natural background. Therefore, we propose to evaluate and show the radon doses of the patients in their medical records in the future. We have also estimated the annual effective dose equivalent from radon and its decay products for the staff members of speleotherapeutic treatments and found that it is probably in the range between 15 and 40 mSv/year. We suggest continuous monitoring of their doses (preferably with personal radon dose meters) making possible to prevent them from receiving higher doses than reasonably acceptable.


PP8

CONTENT OF 226Ra IN TAP AND MINERAL WATERS OF THE REPUBLIC OF CROATIA AND POSSIBLE HEALTH EFFECTS

G. Marovic, J. Sencar

Institute for Medical Research and Occupational Health, Zagreb Department of Radiation Protection, HR-41001 Zagreb, Ksaverska cesta 2, P.O.Box 291, Croatia

The presence of 226Ra in drinking water may directly affect human health, due to its exceptional radiotoxicity. The paper describes the study of 226Ra content in drinking water of Croatia: tap water from the public supply system of several towns in Croatia and bottled mineral water from two mineral water springs. In the samples of tap and mineral water collected over several years 226Ra was determined by alpha-spectrometric measurement after radiochemical separation.

The study showed that 226Ra content for investigated categories of waters are below the levels at which any unacceptable dose due to ingestion would arise. The dose from consumption of bottled mineral water has been estimated and compared to the dose received from public system tap water over the year.



PP9

THE RADON-222 CONCENTRATION IN THE DRINKING WATER AND THE CANCER HUMAN RISK

R. Burkhardt, N. Muntean, I. Mocsy

Medical Center and Health Services and Management, Cluj-Napoca, Romania

The biological effects made by the natural irradiation are difficult to define because of the environmental factors acting upon the people. Radon is a natural radionuclide with a wide spread in the environment and it has an important role among the cancer risk factors. It enters the body by the ingestion of drinking water, food and by the inhalation of the air. The radon from the air comes from the water and it is soluble in the fluids and the grease of the body so it is a potential risk factor for the people.

Here we try to put into evidence the relation between Rn in drinking water and the incidence of cancer mortality in a community of people from the town of Miercurea Ciuc in Harghita county.

Thus we determinate the Rn-concentration from the drinking water of the town. We estimated the gastric internal dose by the "Kahbs" method and we carried out a retrospective epidemiological study out the gastric cancer.

With the results obtained we try to estimate the implication of Rn-222 from the drinking water in the human cancerogeneses.



PP10

RADON CONCENTRATION IN ITALIAN CAVES: SOME ASPECTS OF RADIATION PROTECTION

A.A. Cigna

Societa Speleologica-Italiana, Fraz. Tuffo, I-14123 Cocconato, Asti, Italy

The problem of radon has drawn the attention of many scientists all over the world particularly in the last decade. Obviously the main object of the researches carried out on this argument was the evaluation of the indoor radon concentration because this is, in general, the most relevant source of irradiation from radon for the population. Nevertheless also the caves were considered because the radon concentration in caves may rich sometimes values rather high.

In Italy a number of measurements have been carried out in caves and here the radon concentration recorded for each cave are reported. These are listed beginning from North to South Italy. Also the cave file number is given with the cave name.

Some conclusions on the meaning of these data are also included, in particular with an evaluation of the doses involved by exposure to radon in the caves studied.



PP11

METHODOLOGY OF AMBIENT RADON DAUGHTER MEASUREMENTS

R. Winkler, W. Hofmann and R. Rolle

Institut für Physik und Biophysik, Universität Salzburg, Austria

The radiation doses delivered to the bronchial epithelium upon inhalation of radon and its short-lived decay products are caused primarily by the alpha-emitting radon daughters Po-218 and Po-214. Thus the reliability of any dose estimate for risk assessment purposes depends on the accuracy with which these concentrations can be determined in ambient air.

In the present study, four different measurement techniques will be compared: (I) gross alpha quasi-continuous sampling measurements with a Pylon WL-meter, with varying time intervals between sampling and measurement; (ii) gross alpha grab sampling measurements with a Pylon WL-meter, using a new filter for each sampling period; (iii) spectrometric alpha grab sampling measurements with a filter device and subsequent analysis of the alpha spectra; and, (iv) spectrometric alpha and beta measurements with the Rolle"-meter. This methodological study has indicated that the standard deviations of the radon daughter concentrations are smallest for the spectrometric methods.

In a preliminary study in selected working and living environments, the following parameters were also measured: unattached fractions, activity and mass size distributions, number concentrations, humidity and temperature. Only a complete on-site determination of these physical and environmental factors will permit a reliable dose and risk assessment for inhaled radon daughters.



PP12

DEPOSITION OF INHALED RADIONUCLIDES IN BRONCHIAL AIRWAYS: IMPLICATIONS FOR EXTRAPOLATION MODELING

I. Balashazy 1,2 , W. Hofmann 1 and T. Heistracher 1

1 Institute of Physics and Biophysics, University of Salzburg, Austria
2 KFKI Atomic Energy Research Institute, Budapest, Hungary

The validity of extrapolating rat inhalation data to human conditions depends on the similarities and differences of their nuclide deposition patterns. Statistical analyses of human and rat tracheobronchial morphometry data have revealed distinct asymmetric features of their airway branching patterns, particularly for the monopodial branching structure of the rat lung. Our predictions of particle deposition patterns within asymmetric bronchial bifurcations in human and rat lungs are based on a numerical model for the calculation of airflow and particle trajectories in three-dimensional asymmetric bifurcation models: (I) the Navier-Stokes equations for the air velocity field are solved by a finite difference method, and (ii) trajectories of aerosol particles entrained in the airstream are simulated by Monte Carlo techniques.

The effects of interspecies differences in radionuclide deposition patterns are explored for two typical bifurcation geometries in segmental bronchi (generations 4-5) and terminal bronchioles (generations 15-16) of the human and rat lungs, for inspiration as well as expiration. The observed interspecies differences in localized deposition patterns and related deposition efficiencies demonstrate that the respective asymmetries in airway branching affect the local distributions of deposited radionuclides in bronchial airway bifurcations and, consequently, the applicability of extrapolating carcinogenic risk.



PP13

A NEW METHOD FOR RAPID MAPPING OF THE RADON EMANATION POTENTIAL OF THE SOIL OVER LARGE AREAS

M. Andjelov 1, J. Cloute-Cazalaa 2, M. Janot 2, P. Jovanovic 3, I. Kobal 4, J.f. Pineau 2, P. Zettwoog 5

1 Institute of Geology, Geotechnology and Geophysics, 61000 Ljubljana, Dimiceva 14, Slovenia
2 ALGADE - BP 46 - 87250 BESSINES, France
3 Institute of Occupational Safety of the Republic of Slovenia, 61105 Ljubljana, p.p. 27, Bohoriceva 22a, Slovenia
4 Jozef Stefan Institute, Jamova 39, POB 100, 61111 Ljubljana, Slovenia
5 CERTAC, S.A., France

The method is based on differential gamma spectroscopy with a collimated GeHP gamma detector.

By studying the differential absorption of different gamma lines of the U decay chain, it is possible to obtain the radon profile in the soil under investigation.

The first experiments, conducted in France and in Slovenia, show interesting results, even with a small volume detector.

Further development of this method will be implemented, to allow it to be used on board a truck or an airborne platform.



PP14

RADON IN THE SPAS IN THE REPUBLIC OF CROATIA

N. Lokobauer, Z. Franic, J. Sencar, G. Marovic

Institute for Medical Research and Occupational Health, Zagreb, Department of Radiation Protection
HR-41001 Zagreb, Ksaverska cesta 2, P.O.Box 291, Croatia

The paper deals with the investigation of indoor radon activity concentrations in the following spas in the Republic of Croatia: Bizovacke Toplice, Stubicke Toplice, Tuheljske Toplice, Krapinske Toplice, Varazdinske Toplice and Istarske Toplice.

Radon activity concentrations were measured by means of solid state nuclear track detectors (Kodak LR-115 films). The investigations include indoor measurements around the swimming pools at the levels of 2m and 0.5m above the water surface.

Elevated radon activity concentrations were detected in the spa of Istarske Toplice, which are known as "sulphur radioactive spa". In this spa the average radon activity concentrations measured around the swimming pools at the levels of about 2m and 0.5m above the water surface were 872 Bqm-3 and 926 Bqm-3, respectively.



PP15

DIFFUSION CHARACTERISTICS OF ATTACHED AND UNATTACHED RADON PROGENY OVER A VEGETATED SOIL

V. Cuculeanu and A. Lupu

National Institute of Meteorology and Hydrology, Bucharest, Romania

Assuming steady-state diffusion equation within both vegetation and open atmosphere, the radon/thoron and daughter profiles were deduced using the Green's function method. This analytical approach has the advantage of providing a unique solution for the diffusion equation, thus eliminating the errors introduced by the usual numerical methods.

Gravitational settling has been taken into account using different sedimentation velocities for the attached and free daughters. At the ground level the boundary condition consists in equating the flux due to the concentration gradient and gravitational settling with the deposition rate.

The turbulent diffusion coefficient within vegetation was quantified in accordance with the existing experimental data deduced from the concentration gradients.

The equilibrium factor and the unattached fraction were studied for different turbulence intensities, vegetation types and aerosol concentrations.

The predicted values of concentration, equilibrium factor and unattached fraction were compared with experimental values and a reasonable agreement was noted.



PP16

MEASUREMENT OF THE AMBIENT NEUTRON BACKGROUND WITH A HIGH-RESOLUTION -RAY SPECTROMETER

M. Korun, R. Martincic, B. Pucelj, M. Ravnik

Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia

The fluxes of thermal and fast neutrons were measured by a high-resolution -ray spectrometer. Capture -rays from absorption of neutrons in boron were detected. For the measurement of the flux density of thermal neutrons the sensitive volume of the detector was surrounded by a thin converter (~ 0.2 g cm-2) of boric acid. Fast neutrons were slowed down and absorbed by a thick converter (~ 3 g cm-2) of borated paraffin. The measured flux density of thermal neutrons 1.7 +- 0.8 10-3 cm-2 s-1 agrees well with the published values [1,2], whereas the flux density of fast neutrons 16 +- 3 cm-2 s-1 agrees with the data from [2] and exceeds the value from [3] for a factor of two.

References:

  1. G. Heusser, Nucl. Instr. And Meth., B17 (1986) 418,
  2. G. P. koro et al., Nucl. Instr. And Meth., A316 (1992) 333,
  3. NCRP Report No. 94 (1987), NCRP publications, Bethseda, USA.



PP17

ENVIRONMENTAL-RADIOLOGICAL MONITORING SYSTEM AT MECSEKUR N LTD (MECSEK MOUNTAINS, HUNGARY)

A. Varhegyi, I. Barany, I. Vados

Mecsekuran Ore Mining Ltd., H-7614 Pecs, P.O.B. 65., Hungary

The uranium mining activity has been started in 1956. in Hungary (in Mecsek mountains, Southern part of the country). Since that time, about 20 million m3 rock has been removed, enormous tailings hills and tailings ponds has been produced and the depth of mining exceeded 1000 m. The mining and milling has a significant impact both on the natural and the human environment. To study and manage that impact, a monitoring system has been established and continuously developed on the influenced area.

Air, aerosol, fall-out, water, plant and soil samples are regularly collected for detailed radiological analysis. The natural radioactive nuclide content of samples are analysed both qualitatively and quantitatively with high resolution gamma spectroscopy. The radiological contamination of uranium mining district is controlled by systematic in situ gamma-ray dose, radon concentration and radon exhalation measurements. The surfacial, mine and groundwaters are monitored by regular sampling and subsequent radiochemical analysis (for U, Ra and Rn content). Automatic radon monitoring devices are operated in the dosemetrically most critical points of the mines and mill. The annual activity escape from the mines and mill into the environment is also monitored.



PP18

RADON MITIGATION IN SOILS

D. Ristoiu 1, C.Cosma 1, T. Ristoiu 2

1 University Babes-Bolyai, Cluj-Napoca, Romania
2 Technical University, Cluj-Napoca, Romania

Radon is produced in soil by Radium decay, being an Uranium daughter. Radon mitigation from soil to atmospheric air is due to pressure, concentration and temperature gradients existing between soil and air.

The pressure-induced flow (advection) prevails in fractured soils with crack radius r>0.001mm. The concentration gradients determine radon diffusion from soil to air. Diffusion prevails in porous soils with pore radius r<1um, while in compact soils with a fine granulation, r<0.01um, radon mitigation takes place by Knudsen diffusion. Generally Knudsen diffusion has a small contribution, while advection and diffusion are the main mechanisms of radon mitigation in soils. The existence of temperature gradients is favouring the termodiffusion which appears especially around soil surface.

Radon transport from soil to air is determined by soil parameters as: porosity, granulation, moisture, and it is influenced by meteorological conditions such as: atmospheric temperature and pressure, winds and precipitations.

We developed a theoretical model for simulation of radon mitigation in soil and its dependence of these parameters. We also made an experimental device for verifying the theoretical model.



PP19

SURVEY OF RADON ACTIVITY AT GROUND LEVEL IN VILLAGE HOUSES OF HUNGARY

E. Toth

Lauder School, Budapest, Hungary

In the year 1994/95 over 3000 country houses were measured in Hungary (ground floor, bedroom, pillow level, several seasons) with the help of CR39 track detectors. The distribution shows a lognormal character with high confidence level, indicating several factors influencing the radon concentration indoor. In this way regions with enhanced radon activity concentration could be found. The overall number of houses above international action limits (above 400 Bq/m3, or above 800 Bq/m3 respectively) can be estimated. The survey has been made able by the responsible cooperation of physics teachers and their students countrywide. It has been supported by the OMFB and by the OTKA-T7603 project for buying instruments and detectors.


PP20

EFFECT OF ATMOSPHERIC PRESSURE ON RADON ENTRY RATE INTO HOUSES

A. Vasarhelyi, I. Csige, J. Hakl, I. Hunyadi

Institute of Nuclear Research of the Hungarian Academy of Sciences, H-4001 Debrecen, POB 51, Hungary

We have studied the effect of atmospheric pressure variation on radon entry rate into houses by measuring the radon activity concentration and the air pressure as a function of time in two dwellings. The houses were studied under normal living conditions. From the measured time series, we have selected time intervals, in which the doors and windows of the houses were kept closed continuously. For each of these periods we analyzed the build up of the radon activity concentration, and determined the radon production rate [Bqm-3s-1], and the natural ventilation rate [h-1] of the room. For both houses we assumed that the main source of radon is the underlying soil. According to this, we have estimated the average exhalation rates by dividing the radon production rate by the surface of the floors.

Investigating the average exhalation rates as a function of the atmospheric pressure we have found an anticorrelation between them. We have also observed a hysteresis in the average exhalation rate - pressure curve. Modelling radon entry rate into houses from porous media under varying atmospheric pressure condition we found agreement between theoretical and experimental results.



PP21

CALIBRATION OF A DOSIMETER FOR DETECTION OF RADON ACTIVITY IN AIR

M. Caresana, V. Cattaneo

Dipartimento di Ingegneria Nucleare, Politecnico di Milano, Milano, Italy

The purpose of this work is to illustrate the calibration of an ionization chamber to be used for calibrating dosimeters based on the cellulose nitrate film LR115, produced by Kodak.

The chamber is filled with a radon concentration obtained from a source of few Ci of salts of Ra-226, contained in a cruet; the value of this radon concentration is obtained by drawing a known volume of radon-air blend in a vial and by measuring the activity with a Ge-Li counter, intercalibrated with the Italian Primary Metrological Center. The drawing of gas is made using two different methods, in order to avoid systematic errors due to the radon-air blend movimentation.

The calibration factor of the ionization chamber, namely ratio between the equilibrium current and the radon concentration, is 3,77 1016 Bq/m3/A.

Concerning the dosimeters calibration, is our experience a good exposure time, within the calibrated chamber, of about one or two days.

The calibration factor of the dosimeters in resulted to be 4,7 10-4 tr/cm2/Bq*h/m3.



PP22

DOSE AND RADON MEASUREMENTS INSIDE HOUSES CONTAINING ASH AS BUILDING MATERIAL

R. Bodnar, Z. Lendvai, C. Nemeth, J. Somlai

University of Veszprem, Dept. of Physics, Veszprem, Hungary

The natural radioactivity 238U and its daughter elements in rocks - as in coal resources too - of the Transdanubian region can reach ten to twentyfold of the world average.

After coal processing the derivatives (slag, ash, waste) become enriched in those decay elements even 40-80 times of the world average.

Unfortunately these materials were built in houses - sometimes in offices or schools - as backfill or insulation.

In these buildings partly the dose caused by outer gamma-radiation is rising (on the floors and roofs of these buildings 500-900 nSv/h dose can be detected). On the other hand, the radon concentration depending on the emanation factor of these materials and the way of life is found to be very high (600-2000 Bq/m3), thus the inner radiation dose deriving from that is also significant.

At those places, that have high radon concentration together large dose rate, the achieved dose can only be reduced by costly architectural intervention.



PP23

RADIOLOGICAL IMPACT OF SOME UTILIZATIONS OF THERMAL WATERS FROM THE WESTERN PLAIN

G. Dinca, T. Peic

Research and Design Institute for Rare and Radioactive Metals-Research Laboratory for Radiation Protection, Working Conditions and Ecology- Petru Groza Town, Romania

Natural uranium, radium 226 and radon 222 content of thermal waters springing from 67 wells from Satu Mare, Bihor, Arad and Tim districts and the radiological impact of these due to utilization were investigated, over 1700 radiochemical and radiometric measurement being performed. The mean contents are comparable to those of ground waters, varying only with respect to the area: natural uranium from 0.003 to 0.013 mg/L, radium from 0.02 to 0.10 Bq/L, and radon 222 to 9.5 Bq/L.

At the wells in the perimeter of Oradea city, the thermal water has an uranium content comparable to that of ground water, but the radon content is 4 to 8 times higher and radium reaches to 2.5 Bq/L, the mean value for the 5 wells being 1.4 Bq/L. These thermal waters are used in the swimming-pools from Oradea and also as warm water over the last 10 years period, in about 1400 flats.

It was not proved a radiation risk for public or a pollution of the environment at B ile Felix, B ile 1Mai and Moneasa spas or at the swimming-pools from Carei, Marghita, Satu Mare or at the usage of thermal water as heat source or at flax and hump retting.

The possibility of existing high radium content thermal water sources, enforces the medical licensing for any future utilization.



PP24

RADON-222 CONCENTRATION IN DIFFERENT DWELLINGS FROM CLUJ-ROMANIA

I. Mocsy, N. Muntean

Medical Center and Health Services and Management, Cluj-Napoca, Romania

We studied Rn-222 concentration from indoor air in two types of dwellings: block of flat district (concrete made) and a detached-houses zone (red brick made). These dwellings are different by the building materials, by the type of heating, by their level from the soil and by the surface of the rooms.

Radon concentration was determined in all the rooms under normal living conditions in the period of Sept.-Nov. 1994. The "SI-5S Prassi" apparatus was used for this. The values of Rn-222 from the air in the blocks were between 30-80 Bq/m.c., the maximum values being over 100 Bq/m.c. in the case of non-ventilation within 12 hours.

In the detached-houses under the same conditions, maximum values, higher than 500 Bq/m.c. were found in non-ventilated rooms having no cellars (140-150 Bq/m.c.) as against those with cellar. No significant differences were found either related to the building materials or to the type of heating (central heating and natural gas).

We found of special importance the increased Rn-222 concentrations in the air of the bathrooms after water use.

From the analysis of the results follows that the most important contribution to the accumulation of Rn-222 in the indoor spaces is related to the type of foundation and the soil under the houses.



PP25

THE SPATIAL DISTRIBUTION OF 222RN "INDOOR" IN SLOVENIA AS A STOCHASTIC MULTIFRACTAL PROCESS

G. Salvadori 1, S.P. Ratti 1, G. Belli 1, I. Kobal 2, J. Vaupotic 2

1 University of Pavia, Department of Nuclear and Theoretical Physics, Via A. Bassi, 6 - 27100 Pavia, Italy
2 Jozef Stefan Institute, 61111 Ljubljana, Jamova 39, P.O.Box 100, Slovenia

In this paper we show an original application of the theory of fractals and stochastic multifractals to the analysis of the spatial distribution of 222Rn "indoor" in Slovenia. The data consist of about 1300 measurements collected in schools, in buildings made of wood or concrete.

The dangerousness of Radon may depend upon its in situ concentration, however, the presence of "hot spot" may not be detected due to averaging procedures or to insufficient spatial and/or (fractal) dimensional resolution of the sampling network.

The geometry of the network show fractal features which, in turn, gives a sparse (inhomogeneous) sampling of the phenomenon: this means that some of its components (especially the most intense ones) are almost surely missed in the gaps of the networks themselves. The values of radioactive concentration show an (asymptotic) hyperbolic distribution (a fingerprint of multifractality), revealing the presence of a high variability and of strong local fluctuations.

The application of both the P.D.M.S. and D.T.M. techniques show the presence of (stochastic) multifractal structures; the estimate of the relevant parameters indicates that the spatial distribution of Radon can be classified as a "conditionally soft/hard" multifractal process.

Overall, this research shows that fractals and multifractals represent a powerful tool to characterize the Radon pollution of the environment by means of a single statistical law, from the smallest up to the largest spatial scales, without introducing arbitrary data regularization.



PP26

SCANNING ELECTRON MICROSCOPY OF RAT THROAT AND TRACHEA FOLLOWING THE EFFECTS OF RADON DECAY PRODUCTS

J. Rode #, J. Vaupotic *, K. Draslar v, I. Kobal *

# Institute of Biology, Ljubljana, Slovenia
* Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia
v Department of Biology, Faculty of Biotechnology, Ljubljana, Slovenia

In two preliminary experiments, laboratory rats were exposed in a small chamber (0,25 m3) to radon-rich air. In both experiments the exposure was about 0.9 WLM. In the first run two rats were exposed for 14 days and in second one three rats for 6 days. In the throat and trachea of the rats the effects of radon decay products were followed by scanning electron microscopy.


PP27

RADIATION DOSE ESTIMATES IN SLOVENIAN KINDERGARTENS APPLYING SOLID STATE DETECTORS

J. Vaupotic, I. Kobal

Jozef Stefan Institute, Jamova 39, 61111 Ljubljana, POB 100, Slovenia

In the radon survey programme in kindergartens in Slovenia, instantaneous indoor air radon concentrations were obtained under closed conditions in all 730 such buildings using alpha scintillations cells. At each place one room was selected for inspection. In all these rooms the gamma dose rate was also recorded with a portable scintillation instrument. In 50 places in the city of Ljubljana with radon concentrations more than 200 Bqm3, track etch detectors and thermoluminescent dosimeters were exposed for three months in winter time in order to obtain average indoor radon concentrations and gamma dose rates, respectively. An average ratio of the average concentrations versus instantaneous ones was obtained, even though this ratio differed substantially from place to place. On the basis of this ratio, radiation doses due to radon and its progeny were estimated for children and personnel in all the kindergartens. Gamma doses were also evaluated.


PP28

GUIDLINES FOR TREATMENT OF SOLID WASTES WITH ENHANCED NATURAL RADIOACTIVITY IN POLISH COAL INDUSTRY

B. Michalik, S. Chalupnik, J. Skowronek, J. Lebecka

Central Mining Institute, Katowice, Poland

In Polish coal mines there are some waste materials of high radioactivity. Enhanced natural radioactivity of these wastes is caused by saline waters which often contain radium isotopes and barium ions. From such waters radium and barium are coprecipitated out by sulphates in underground workings or on the surface. Radioactive deposits sometimes cause radiation hazard for underground crews, serious technical problem in exploitation of pumps and pipelines and radioactive contamination on the surface, mainly in the vicinity of settlement ponds and alongside the river banks. Deposit of RaSO4 + BaSO4, in which concentration of 226Ra may reach even 400000 Bq/kg, sometimes are a source of radiation hazard for mining crews. Elevated radiation doses may be obtained mainly during cleaning of gritters, settlement tanks and storage of radioactive deposits.

Radioactive wastes cause also contamination of the natural environment. Radium and barium sulphates are sometimes precipitated in settlement pond and rivers. Moreover, from radium-bearing waters which do not contain barium ions, radium can be removed from water by adsorption on bottom sediments in rivers. Concentration of 226Ra in such sediments is usually lower than 1000 Bq/kg, but enhanced radium concentrations were found many kilometres from the discharge points.

It was necessary to prepare guidelines for treatment of materials with enhanced natural radioactivity. Such guidelines have been worked out during past few years and applied in all coal mining industry. On the other hand, it is a common practise in Poland, that ashes from power plants are stored underground and such guidelines are also very useful for this purpose.



PP29

QUALITY ASSURANCE SYSTEM IN GAMMA SPECTROMETRY LABORATORY

A. Mielnikow, B. Michalik, S. Chalupnik, J. Lebecka

Central Mining Institute, Katowice, Poland

On basis of guidelines for development of QUALITY SYSTEM for a testing laboratory (European Norm Series EN 45000) a quality assurance system was implemented in gamma spectroscopy laboratory, where routine measurements of natural (mainly Ra-226, Ra-228, Ra-224, K-40) and artificial (mainly Cs-137 and Cs-134) isotopes are performed. We measure a variety of samples, but mainly coals, rocks, ashes, deposits, vegetation and air filters.

Laboratory of gamma spectroscopy in Central Mining Institute has three HPGe detectors. There is one coaxial detector with 45% relative efficiency, one detector for low energy region and one detector with extended range). We have also two Ge(Li) detectors from former Czechoslovakia. Shielding is made of steel - with thickness 40 cm. The electronics and software (Genie-PC) was bought at "Canberra" and "Silena".

The paper describes not only the system of quality assurance but also main problems met by its implementation and results of intercomparison measurements. The QAS has been introduced in 1992. In 1993 the Accreditation Certificate of Testing Laboratory for our Laboratory has been obtained from the Polish Bureau of Research and Certification as a fifth laboratory in Poland.



PP30

EQUIPMENT FOR THE OPTICAL EVALUATION OF NUCLEAR TRACK DETECTORS

N. Vana and P. Hofmann

Atomic Institute of the Austrian Universities, Schüttelstrae 115, A-1020 Wien, Austria

The equipment for nuclear track evaluation consists of a microscope, a video camera and a PC. With the software of the video-digitizer track dimensions and their mean grey value can be measured on the monitor with a resolution about 0.27 um.

This equipment has been used to evaluate MAKROFOL and CR-39 detectors which were exposed in space on the MIR-space station for several months.

This equipment was also used for thermal neutron-dosimetry with a lower limit of 0,5 mSv/cm2, alpha particle measurement and measurement of the fluence of 12C ion beams in the Dubna synchrophasotron.



SESSION III:
RADIATION PROTECTION AND ENVIRONMENT


OP18

KRSKO NPP ECOLOGICAL INFORMATION SYSTEM

A. Kovac, B. Breznik

Nuklearna Elektrarna Krsko, 68270 Krsko, Slovenia

Krsko Nuclear Power Plant Ecological Information System (EIS) was developed for two main functions.

The first function is to collect data from different measuring points, proceed the data and distribute them to some places at power plant and to some outside institutions. EIS collects data from three automatic meteorological stations, hydrological station on Sava river, some continuous dose rate measuring devices located in the vicinity and from Radiation Monitoring System.

The second function of EIS is dose calculation in case of emergency. Dose calculating programme is important part of EIS and with its calculations and graphical displays offers tool and support for dose assessment.



OP19

TRITIUM MEASUREMENT BY GAS SCINTILLATION

F. Campi, C. Mascherpa, S. Terrani

Nuclear Engineering Dept., Polytechnic of Milan, Italy

For civilian purposes Tritium is presently used in quantities of tens of PBq (MCi) in laboratories for the studies of technology involving Tritium, at the JET plant as fuel for the process of nuclear fusion and in the manufacture of radio-luminescent items.

Given the extreme mobility of Tritium in most materials, it is necessary to use systems for double containment, such as glove boxes or spaces between primary and secondary container, in which inert gas like argon or nitrogen flows. With these systems it is possible to recover Tritium that escapes from the primary containment. Presently the gas flow is monitored continuously by means of ionization chambers which may present problems in particular applications ("memory effect" with high activity, strong dependence of the response on the presence of impurity, etc.).

The aim of the work presented is to determine the prospects for realizing a new type of monitor principally dedicated to measuring the gas activity in the isolation spaces of the containing systems of the high activity Tritium plants. This monitor should have sufficient sensitivity, quick response and should be easily decontaminated.

As detection technique we chose the scintillation produced in the inert gas by radioactive decay. With the first prototype, designed in cylindrical form, it was possible to observe gaseous scintillation events in mixture of Tritium and argon or nitrogen. Following that, a spherical prototype was designed of which we studied the performances and the dependence of the response varying the pressure, the concentration of Tritium, the percentage of the impurity and the gas flux.

The results are satisfactory and suggest that the monitor could be used in glove boxes and double containment systems. In the future we plan to test the monitor using large quantities of Tritium and to study the dependence of the response on the size and shape of the monitor chamber.



OP20

EVULATION OF LOW-LEVEL SOLID RADIOACTIVE WASTE GENERATED BY A LARGE HOSPITAL AND DISPOSED OF WITH ORDINARY REFUSE

L. Conte, G. Pedroli *, M. Monciardini, R. Novario, A. Beretta

Servizio di Fisica Sanitaria dell'Ospedale di Circolo di Varese, Italy
* Servizio di Fisica sanitaria dell'Ospedale S. Gerardo di Monza, Italy

Radioactive waste is an inevitable result of the use of unsealed radionuclides in Nuclear Medicine. There are three types of waste: liquid, solid and gaseous. Solid waste usually consist of used generators, contaminate glassware, syringes, cleaning material, bench cover and so on. Material which cannot be disposed of immediately shall be stored for decay level which permit disposal with ordinary refuse. Solid waste, such as contaminated paper, glassware, swabs and similar material may be immediately disposed of with an appropriate volume of ordinary refuse.

The activity of these low-level solid radioactive waste was monitored to estimate the fraction of the employed activity of the solid low-level waste generated in different practices which concern the use of unsealed radioactive substances in therapy, diagnosis "in vivo" and "in vitro".



OP21

MODELLING THE CHERNOBYL RADIOACTIVE FALLOUT IN EUROPE: A MULTIFRACTAL APPROACH

G. Salvadori, S.P. Ratti, G. Belli, E. Quinto

Universita degli Studi di Pavia, Dipartimento di Fisica Nucleare a Teorica, Via A. Bassi 6, I-27100 Pavia, Italy

This work deals with the 137Cs cumulative soil deposition in several European Countries. The measurements, collected after the Chernobyl nuclear accident, come from the REM data bank and amount to a few hundred samples. We study both the geographical and the statistical distribution of the measurements, showing the existence of an (asymptotic) hyperbolic behaviour as well as the presence of multifractal features. Based on such analyses, we introduce a multifractial model to describe the overall distribution of the radioactive pollutant, even in sites where no data are available. Our working hypothesis is that the fallout is strongly influenced by complex meteorological factors, which are known to feature fractal properties.


OP22

OFF-SITE EMERGENCY PLANNING IN CZECH REPUBLIC

Z. Prouza

Centre of Radiation Hygiene NIPH, Prague, Czech Republic

The principles of emergency planning in the Czech Republic are based on the same philosophy as the ICRP Publication 40 and the IAEA Safety Series No. 55 and 72, and include already the post Chernobyl experiences. The Czech Republic legislation, in connection with political and economical changes in the country, experiences an extensive reconstruction and proposals of the Law on "Peaceful Use of Nuclear Energy and Ionizing Radiation" ("Atomic Act") and Act on "Prevention and Liquidation Industrial Accidents and Natural Catastrophes" already being elaborated. These Acts and related laws should solve our legislative problems on field of emergency planning and preparedness. The structure, philosophy and principles of the proposal of the "Atomic Act" will be built on new International Basic Safety Standards.

At the present time our regulations are based on an assumption that the protection measures (PM) are introduced in the cases where it is to assume that intervention levels (IL) will be exceeded. When exceeding the upper limit of the IL interval for given PM, the implementation of that PM is regarded as necessary, when the lower limit of the IL interval is exceeded, the optimization is provided with respect to the extent, feasibility and price of the given PM.

Principles of protective measures implementation in the case of an occurring or suspect radiation accident (several PM are carried in Emergency Planning Zone after warning and without waiting for result of monitoring the actual radiation situation and without waiting for a decision of District Emergency commission, the others are implemented in agreement with results of monitoring, actual course of accident and on the decision of District Emergency Commission) are explained. Present the emergency planning structure in Czech Republic is demonstrated.



OP23

RAPID DETERMINATION OF SOIL CONTAMINATION BY HELICOPTER GAMMA RAY SPECTROMETRY

I. Winkelmann, H. Buchröder, M. Thomas

Bundesamt für Strahlenschutz, Waldowallee117, 10318 Berlin, Germany

Nuclide specific aerial measurements of surface soil contamination were performed after the Chernobyl reactor accident in the southern part of Germany. For these measurements, a helicopter equipped with a gamma ray spectrometer system including a HPGe detector (50 % relative efficiency) and 3 NaI(Tl)-detectors (volume 12 l) was used. The paper describes the complete measuring system in detail which can be used for nuclide specific measurements of soil contamination as well as for the detection of sources of gamma radioactivity. At an altitude of 100 m, a soil contamination of several kBq/m2 for 134Cs and 137Cs can be measured with a HPGe-detector by a measuring time of 60 s (helicopter speed 100 km/h). For the detection of gamma rays emitting point sources, the 12 l NaI(Tl)-detector is used. Assuming line spacing of 300 m and a speed of 100 km/h, an area of about 30 km2 can be surveyed per hour. Thus 60Co-sources of some GBq activity can be detected. The system was practically applied the first time by measuring the deposition of artificial radionuclides in the southern part of Germany after the Chernobyl reactor accident. The aerial measuring system was also tested in the former USSR, in a region north of Chernobyl, with nuclide deposition values of up to 2MBq/m2. The results of aerial measurements in selected areas are presented.


OP24

RECENT DEVELOPMENTS IN THE ATMOSPHERIC DISPERSION MODELS TO BE USED FOR REGULATORY PURPOSES AND IN RISK EVALUATION

G. Graziani

Environment Institute, JRC Ispra, 21020 Ispra, Italy

This paper presents some of the recent improvements introduced in the regulatory dispersion models. In particular, the classical Pasquil-Goffered parameterization of atmospheric turbulence is abandoned, as it has been warmly suggested by the scientific community during the three Workshops on this argument that were held over the last two years in Europe (Risoe, Denmark, May 1992; Manno, Switzerland, August 1993; Mol, Belgium, November 1994). The alternative is the use of similarity theory with the definition of physical quantities, such as the Monin Obukhov length and the friction velocity, that vary with continuity. These quantities can be determined from a few meteorological measurements that are usually available at the foreseeable release sites of conventional pollutants. The dependence from these quantities of the turbulent parameters, like dispersion coefficients and mixing layer depth is also reported.

As a further improvement, a recent solution of the dispersion equation is also given that takes explicitly into account the finite emission duration.



OP25

BIOPHYSICAL MODEL FOR THOROTRAST-INDUCED LIVER CANCERS

M. Nösterer 1 , W. Hofmann 1 and S.G. Andreev 2

1 Institute of Physcis and Biophysics, University of Salzburg, Austria
2 Institute of Chemical Physics, Russian Academy of Sciences, Moscow, Russia

Between 1930 and 1950, an estimated 10,000 to 20,000 patients received Thorostrast injections in Germany. About 59% of the intravascularly injected Thorotrast was retained by the liver. Based on a mean injected volume of 25 ml and an average exposure time of about 40 years, Thorotrast patients received a mean liver dose of about 9 Gy. As a consequence, 35% of German Thorotrast patients died of liver tumors; in contrast, no case of primary liver tumors was observed in the control group.

A biophysical model for Thorotrast-induced liver carcinogenesis has been developed, which is based on experimentally observable in-vitro cellular radiation effects, such as cell killing, oncogenic transformation, stimulated mitosis, removal from contact inhibition and adaptive response. In this initiation-promotion model, we assume 7 transitions in the development of a cell from the initial unirradiated level (state 0) to a fully transformed cell, eventually leading to a frank tumor (state 7).

Consistent with the epidemiological evidence provided by the German Thorotrast study, our biophysical model predicts that (I) the cumulative incidence rises steeply with increasing cumulative exposure after a mean latency period of about 20 years, and (ii) a higher dose rate leads to a higher cumulative incidence at the same cumulative exposure time, but to a lower incidence at the same cumulative dose ( inverse dose-rate effect").



OP26

MONITORING OF NATURAL RADIOACTIVITY IN SLOVAKIA

D. Nikodemova, M. Vladar, I. Gomola

Institute of Preventive and Clinical Medicine, Bratislava, Slovakia

The aim of the work was to determine the average effective dose to the Slovak population from external radiation and radon daughter inhalation. This estimation has been done by experimental procedures.

The effective dose after external irradiation summarizes contributions of cosmic and terestial components of natural radiation. The territorial net of thermoluminescent detectors and monitoring net IRIS were used for this purpose.

Screening of the equilibrium equivalent radon concentration (EER) in randomly chosen dwellings of Slovakia was used as a basis for the estimation of the population effective dose due to radon inhalation. For EER estimation an integral method using the solid state track detectors was applied.



OP27

EFFECT OF DIFFERENT TREATMENTS ON 110mAg PLANT UPTAKE IN VARIOUS SOIL TYPES

P. Szerbin and E. Koblinger-Bokori

"Frederic Joliot-Curie" National Research Institute for Radiobiology and Radiohygiene, POB 101, Budapest, 1775, Hungary

110mAg contamination of the environment may occur as a result of atmospheric release during normal operation of nuclear power plants (NPP). There is some data, according which the 110mAg release of NPPs, equipped with soviet-type WWER reactors, such as the NPP Paks, Hungary, increase in the early periods of operation. Besides, considerable amount of 110mAg was released to the atmosphere during the Chernobyl reactor accident.

Stable silver generally is not an important pollutant, therefore very few references are available on plant uptake of silver, the same is true for the radiosilver studies.

In the presented study plant (yellow leguminous bean) uptake of 110mAg from different types of soil was investigated. Most typical Hungarian soils (leached Ramann brown forest soil, alluvial soil, chernozem-light sandy soil, calcareous chernozem soil) were selected for the experiments carried out under laboratory conditions. Results are presented in relation to major soil characteristics and, in addition, effects of two different treatments: phosphate and organic matter fertilization on plant uptake are given.

The highest uptake was found in bean grown on leached Ramann brown forest soil, whereas the lowest value was measured in the plant grown in calcareous chernozem soil. Organic fertilization reduced significantly the uptake of radiosilver in all investigated types of soil. The largest factor of reduction was found to be as high as 5. Phosphate fertilization was less effective.

Our study clearly demonstrates that carefully selected post-accident treatment (e.g. organic fertilization following silver contamination) can significantly reduce the environmental consequences of radioactive release. Methods to be developed on the basis of such studies, could be used for remedial actions of agricultural lands, polluted with radioactive substances.



OP28

A FIVE YEAR , POST CHERNOBYL ACCIDENT, SURVEY OF CS-137 LEVEL IN SOME ROMANIAN FRESHWATER BASINS

S. Salagean, C. Fulea, I. Mocsy, I. Uray, N. Muntean

Medical Center and Health Services and Management, Cluj-Napoca, Romania

During the period between 1987-1991 there were prelevated water, seston and sediment samples from two dam lakes - Gilau (Cluj county) and Virsolt (Salaj county) and from the river Somes - representing the drinking water sources of the riverside population.

The Cs-137 content from water was determinated radiochemical with Ammonium Phosphomolybdate, and for the seston and sediment samples there were made gamma-spectrometric analyses with a multichannel analyzer.

The presence of Cs-137 was still detected in all the investigated samples and in all the stages of prevelation, five years after the Chernobyl nuclear accident.

The distribution of Cs-137 was as follows: 92.61 % to 99.60% in sediment, 0.32 % to 7.33 % in seston and under 1% in water. This demonstrates a massive accumulation in sediment, with values of the K.D. (distribution coefficient) up to thousands. At the same time a concentration occurred on the level of the physical and biological supports from water, which was proven by the high values (between 5 and 180) of the F.C. (concentration factor) of Cs-137 in seston. This accumulation has a special importance, because "the stocking" of the radionuclide from water-diminishes the environment and population's contamination risk.



OP29

RADIOACTIVE WASTE REPOSITORY AND RADIATION PROTECTION

M. Stepisnik, O. Jarh, I. Mele

Agency for Radwaste Management, Hajdrihova 2, Ljubljana, Slovenia

Radioactive waste in Slovenia comes not only from nuclear power plant Krsko but also from industry, hospitals and research. These wastes can potentially present risks to health and environment if they are not managed adequately. The Agency for Radwaste Management is responsible for providing the final disposal of radioactive wastes in Republic of Slovenia. Since most of the waste is categorized as low and intermediate level - short lived waste (according to IAEA classification) the work is oriented towards the construction of LILW repository. It must guarantee complete isolation of radionuclides for a period of 300 years. By this time the activity of radionuclides will decay to a level comparable to natural radioactivity of environment.

The site selection criteria has been established but the decision about the location for final repository in Slovenia is not yet made due to strong public opposition. Environmental studies and research work on environmental impact of different disposal types as well as the survey of international practice were carried out. We are strongly aware of extreme importance of radiation protection at future repository site in Slovenia. The preparation of the program of initial state measurements is in the final phase and will provide the reference data for future environmental monitoring at the time of operation of the repository. The preliminary study of acceptance criteria for low and intermediate level radioactive wastes deals with criteria that radwaste should meet in order to minimize the public exposure, to enhance environmental protection and to optimize the economy of waste management. Future studies must prove full safety of repository in compliance with our legislation.



OP30

NUCLEAR DISASTER MANAGEMENT THE MURMANSK EXERCISE

C. Schmitzer

Austrian Research Centre Seibersdorf, Austria

Jointly initiated by NATO Partnership for Peace and UN Department for Humanitarian Affairs, the EXERCISE '95 took place on the Kola peninsula near Murmansk, Russia. Organised by the Russian ministry for disaster management, the trigger incident was supposed to be an explosion in a nuclear power plant, similar to the Chernobyl incident.

Different international teams participated in an effort to determine the extent and implications of the incident, gauge radiation levels in the environment, study relief and evacuation procedures, and estimate the applicability of recommended protection measures.

The exercise was organised in three time scenarios, starting with the third day after the accident up to one month after the accident.

The system developed by the Research Centre and employed by the Austrian NBC defence group encompasses a scenario analysis tool based on three-dimensional dispersion calculations and forecasting capability, GPS-based acquisition of radiation data by mobile teams, and permanent site monitoring instrumentation. Additionally, a robust NaI food stuff probe ensures local consumption to be free of contamination.

Information on the general exercise and procedures is given and the Austrian system and its application throughout the exercise is discussed.



PP31

ACTIVITY LEVELS OF CS-137 AND K-40 IN THE GASTRO-INTESTINAL TRACT OF A COW

H. Rabitsch *, E. Pichl *, J. Pletz **, G. Kahr *

* Abteilung für Strahlenphysik, Institut für Theoretische Physik, Technische Universität Graz, Petersgasse 16, A-8010 Graz, Austria
** Fachabteilung fr Veterinärwesen der Steiermärkischen Landesregierung, Graz, Austria

In comparison to single exposures it is of particular interest to study the distribution of radionuclides in the body of domestic animals after continuous ingestion of radionuclides. We performed a study to determine the activity concentrations of Cs-137 and of the naturally occuring K 40 throughout the gastro-intestinal tract of a cow.

As a consequence of the fallout following the Chernobyl accident the cow ingested chronically heavily contaminated forage during four years. The cow was slaughtered in November 1992 and samples of the whole gastro-intestinal tract were taken. The activities of the contents from the forstomachs and the guts were determined immediately after sampling. Other samples of tissues and organs from the tongue along to the rectum had to be deep-frozen and were thawed and prepared before measuring.

Activities of Cs-137 and K-40 were determined simultaneously by gamma counting with the help of semiconductor-detectors.

The activity concentrations of Cs-137 are in general higher than the corresponding concentrations of K-40. High values of the Cs-137/K-40-ratio were obtained for the mucosa of the reticulum, the tongue and the wall of the rumen. Low ratios were found for the activities of the contents in the rumen.



PP32

MODELLING THE CHERNOBYL RADIOACTIVE FALLOUT IN NORTHERN ITALY: A MONOFRACTAL APPROACH

G. Salvadori, S.P. Ratti, G. Belli, E. Quinto

Universita degli Studi di Pavia, Dipartimento di Fisica Nucleare e Teorica, Pavia, Italy

This paper deals with the 137Cs concentration in air/air dust after the Chernobyl nuclear accident in Northern Italy. Measurements from the REM data bank provide the experimental starting point; we exploit here the empirical parametrization of the temporal trend of the radioactive pollution in a few Provinces we calculated in other works. Since the fallout was strongly influenced by complex meteorological phenomena featuring fractal properties, the high space-time variability of the radioactive concentration is modelled by means of fractals, which may also take into account the geographical sparseness of pollution. Here we present an original fractal approach to the overall description of the radioactive pollution, even in sites where no data are available. The model is based on the Fractal Sum of Pulses theory involving additive stochastic processes. The results are interesting, since realistic scenarios of environmental pollution are produced and the quantitative comparisons with the available data are always acceptable for all the sites considered and for the whole time period of interest.


PP33

RADIATION MONITORING NETWORK OF THE CZECH REPUBLIC

D. Drabova, I. Malatova, Z. Prouza, I. Bucina

Centre of Radiation Hygiene, National Institute of Public Health, Prague, Czech Republic

Radiation Monitoring Network of the Czech Republic (RMN) was established after the Chernobyl accident. It consists of laboratories and monitoring groups of hygienic service, nuclear power plants, hydrometeorological service, research institutes and other institutions.

The radiation situation is controlled in principle by three subnetworks in which some or all above mentioned components of RMN participate:

  1. Network of Measuring Points of Air Contamination (MPAC) network has two principal functions - continuous measurement of gamma dose rate (early warning system) on 50 stations on-line connected to the central computer in the Centre of Radiation Monitoring Network in Prague. - continuous aerosols and iodine sampling by high volume air samplers with changing of filters once a week and fallout sampling with sampling period of one month.
  2. Territorial TL-dosemeters network - 202 measuring points distributed on the whole territory of CR. The monitoring interval is in normal situation 3 months.
  3. Network of 12 laboratories with the possibilities for gamaspectrometric and radiochemic analyses of all components of the environment which provide the data concerning the specific activity of radionuclides in various environmental entities. In case of a nuclear accident the system would use also mobile monitoring units.



PP34

THE EFFECT OF MORPHOMETRIC SCALING ON DEPOSITION AND CLEARANCE OF INHALED RADIONUCLIDES

R. Bergmann 1 , W. Hofmann 1 and L. Koblinger 1,2

1 Institute of Physics and Biophysics, University of Salzburg, Austria
2 KFKI Atomic Energy Research Institute, Budapest, Hungary

The linear dimensions of present lung models are based on morphometric measurements on fully inflated lungs. To simulate deposition of inhaled radionuclides in human lungs under normal breathing conditions, airway diameters and lengths have to be scaled down to the smaller dimensions at functional residual capacity. Two scaling procedures have been applied here: (I) all linear dimensions vary with the cube root of the total lung volume, and (ii) the airway lengths remain invariant with total lung volume, while the relative changes of airway diameters increase with progression through the airway system.

Deposition and mucociliary clearance of inhaled particles in a stochastic morphometric model of the human lung are simulated by the Monte Carlo code IDEAL-4. The effects of different scaling procedures on total, regional and local deposition of inhaled radionuclides have been investigated for different particle sizes and breathing patterns. The corresponding effects on the retention patterns of inhaled radionuclides in bronchial airways are illustrated here for two radionuclides: Tc-99m (half-life of 8 days), and J-131 (half-life of 0.25 days).

In general, the various scaling procedures (I) increase total, bronchial and acinar (only for intermediate particle sizes), and (ii) increase retention in bronchial airways, relative to the corresponding simulations based on the original morphometric data.



PP35

RADIOACTIVE FALLOUT NUCLIDES IN A PEAT-BOG ECOSYSTEM

G. Pausch 1, W. Hofman 1, F. Steger 2 and R. Türk 3

1 Institut für Physik und Biophysik, Universität Salzburg, Austria
2 Institut für Strahlenschutz, Forschungszentrum Seibersdorf, Austria
3 Institut für Pflanzenphysiologie, Universität Salzburg, Austria

In the years following a fallout event, the initial contamination pattern will be modified by environmental/biological factors and by human activities. A peat-bog, however, is a special example of an ecosystem, which is generally not disturbed by human activities and in which the soil structure is not affected by animal activities. In addition, lichens, mushrooms and mosses, which typically can be found in a peat-bog, are known to accumulate radioactive fallout nuclides very efficiently and may, therefore, be used as biological indicators of the radioactive contamination.

In the present study, Cs-137 activities from the Chernobyl fallout were measured in the different components of a peat-bog ecosystem in Koppl near Salzburg, together with soil parameters, such as humidity, density and pH-value. The measured samples displayed a wide range of Cs-137 activities (in kBq per kg dry weight): 1.2-11.3 (lichens), 2.4-6.2 (mosses), 1.9-99.8 (mushrooms), 0.8-5.3 (berries), 0.3-11.1 (higher plants), and 0.2-1.5 (bark). From the measured Cs-137 activities in different soil layers (the Cs-137 activity decreases in a linear fashion with increasing depth), surface contaminations in the range of 16.7-28.7 kBq/m2 could be derived. These values compare favourably with the soil contaminations obtained from in-situ gamma spectrometry, based on the measured activity-depth distributions.



PP36

MEASURES OF PLUTONIUM IN ENVIRONMENTAL SAMPLES

F. D Alberti, L. Risposi

Dept. of Physics, University of Milan, Italy

The aim of this work is to study the behaviour of plutonium (Pu-238, Pu-239, Pu-240) in the environment around the Joint Research Centre of Ispra site.

After the International Moratorium in 1963 no release of plutonium in the environment had happened but the burn up of satellite Snap 9A in April 1964, therefore the plutonium concentration in air and in fallout samples has continuously been decreasing, so it was necessary to carry out techniques for the optimisation of instrumentation in order to obtain a better sensibility.

Due to the low activity in the environmental samples, long time measurements are necessary. For this reason solid state detectors were used instead of ionization chambers, because the former gives more stability. By this device sensibilities of the order of 10-5 Bq.m-2 in fallout, of 10-6 Bq.g-1 in soil and of 10-8 Bq.m-3 in air, were obtained. In this work correlations between atmospheric parameters and concentration of plutonium in the samples were considered.



PP37

THE APPLICABILITY OF LICHENS AS RETROSPECTIVE BIOMONITORS OF THE RADIOACTIVE CONTAMINATION IN A MOUNTAIN ECOSYSTEM

M. Gastberger 1 , W. Hofmann 1 and R. Türk 2

1 Institut für Physik und Biophysik, Universität Salzburg, Austria
2 Institut f¨r Pflanzenphysiologie, Universität Salzburg, Austria

Previous studies have demonstrated that lichens are suitable and inexpensive biological detectors of the local nuclear fallout pattern. Particularly in mountainous regions, the deposited radionuclide activities may vary considerably from site to site due to specific local meteorological conditions, which may also affect the growth of lichens and their uptake of radionuclides. Thus the goal of this study was to find out, whether lichens are still suitable biological detectors of the local radioactive contamination pattern several years after the initial deposition event.

In this study, soil and lichen samples were collected from the Stubnerkogel in the Gastein valley, in the south of the Province of Salzburg, Austria. The samples were taken in the summer of 1993, i.e. more than 7 years after the Chernobyl nuclear accident. The measured lichen and soil samples had Cs-137 activities between 400 and 5000 Bq per kg dry weight.

The results of our study suggest that lichens can be used as retrospective biomonitors of the radioactive contamination even a few years after the fallout event. However, the initial contamination pattern of lichens may be modified by several biological factors in the years following the radioactive fallout. Hence, only lichens from sites with similar growth conditions should be considered.



PP38

SOME ASPECTS OF CESIUM DEPOSITION IN TRANSILVANIA (ROMANIA)

C.Cosma, I.Pop, C.Micu and I. Cosmuta

Faculty of Physics, University Babes-Bolyai, Cluj-Napoca, Romania

After the Chernobyl accident there is a large diversity of 137Cs deposits in different countries. In Romania the greatest deposits are on the NE-SW direction, some of these presenting over 20 kBq.m-2 for 137Cs [1].

Our measurements were made using a NP 424 type of four channels gamma analyzer coupled with a large NaI(Tl) scintillator (76x45 mm). The calibration of this installation was made in two different ways: a) by simulation of a volumetric sample using a 137Cs punctual source and b) using romanian standard samples prepared in the frame of the Environmental Radioactivity seminar.

The measurements made using undisturbed soil samples give values between 4-60 kBq.m-2 and show an accumulation of cesium at the base of the slopes.

Following a determination of 137Cs from a roof deposit sample of Cluj-Napoca city also using the gamma spectra obtained immediately after Chernobyl disaster we estimated the other deposit as: 95Nb, 103Ru, 125Sb, 144Ce, 131I, 140Ba, 129Te. For the total contribution in this region we obtained 1.130 kBq.m-2 much larger than the average in Romania.

Reference:
[1] C.Cosma et al.,Studia Universitates Babes-Bolyai, Physica,33(2),65(1988).



PP39

ANALYSIS OF RESPONSES FROM AN ENVIRONMENTAL AIR MONITORING SYSTEM

A. Feher 1, P. Zagyvai 1, L. Nemes 1, H. Bitt 2, K. Kautny 2, S. Vinkovics 2

1 Technical University of Budapest, Institute of Nuclear Techniques, Hungary
2 Bitt Technology, Spillern, Austria

The AMS-01 air monitoring system has been designed for field applications. It operates with two subsequent static filters for airborne particulate and iodine species in order to deliver an early warning if the appearance of artificial radioactivity in the air is confirmed. Gamma counts of contaminating radionuclides are evaluated upon unfolding the contribution of natural radioactivity. This task is rather sophisticated since the quantity of natural radionuclides shows regular seasonal and diurnal fluctuations and rapid occasional changes due to local meteorological effects. The sensitivity of the system is primarily determined by the ratio and the absolute amounts of radon and thoron descendants. Analytical equations describing their build-up and sorption equilibrium on the surface of the particle filter are introduced as they are applied in the evaluation algorithm of AMS-01. Practical solutions are presented which provide an optimal operation with sufficient sensitivity (< 50 mBq/m for 137Cs and 131I) and exemption from false warnings at the same time. Operational experiences as well as methods for testing and calibration are summarised.


PP40

INTERNAL CONTAMINATION FOLLOWING THE CHERNOBYL NUCLEAR REACTOR ACCIDENT

C. Dumitru, M.A. Puscalau

Institute of Atomic Physics, Institute for Physics and Nuclear Engineering ( LAB.7 ), Bucharest-Magurele, P.O.BOX MG-6, Romania

Following the Chernobyl nuclear reactor accident on 26 April 1986, the deposition densities, in Bucharest area, were 47 kBq/m2 for I-131, 4.3kBq/m2 for Cs-134 and 9.0 kBq/m2 for Cs-137. Iodine-131 was measured in human thyroid since 12 May 1986 till 17 June 1986, for 390 adults residing in Bucharest. Cs-134 and Cs-137 body contamination was measured in 2883 adults (1656 males and 1227 females) from July 1986 and December 1989.

Both measurements were made using a Whole Body Counter, equipped with a NaI(Tl) thyroid detector and a NaI(Tl) body detector.

From the activity, experimentally determined, we calculated the beta and gamma equivalent dose in thyroid, using the 364 key peak-area of the Iodine- 131. For the measurement period, this was 1635 uSv, compared with 2800 uSv thyroid equivalent doses reported for Romania to the United Nations of Scientific Committee (1988) Fig.XVI.

For Cs-134 and Cs-137, we calculated the effective doses, separately. In the period from May 1986 till December 1989, the total effective dose accumulated from intake of Cs-134 and Cs-137 was 352.3 uSv, from which 150.6 uSv was the contribution of Cs-134 and 201.7 uSv was the contribution of Cs-137, values which are in accordance with effective doses values reported for Romania ( Bucharest area ) to the United Nation Scientific Committee (1988) Table 20.

The correlation between body burden with these radionuclides and food consumption is also described.



PP41

THE CONCENTRATION OF RADIOACTIVE STRONTIUM AND TOTAL STRONTIUM IN SOME SAVA RIVER SAMPLES

K. Kosutic, Z. Grahek, S. Lulic

"Rudzer Boskovic" Institute, Center of Marine Research, Bijenicka 54, Zagreb, Croatia

The presence of inactive and radioactive strontium in the effluents and their possible interactions in environment are of a special radiological interest. The physicochemical state in which particular radionuclides are found is important for the uptake of radioactive substances into organisms. The parameter of the circulation of strontium in a biological chain is the "concentration factor" which indicates the possibility of accumulation radioactive strontium in particular biological species.

The objective of this paper is determineted radioactive strontium (90Sr), total calcium and total strontium in the samples of the Sava river (water, sediment and some species of fishes), to calculate the values of "concentration factor" parameter.



PP42

RADIOACTIVE CONTAMINATION OF ANIMAL BONES BY 90Sr

Z. Franic, M. Maracic

Institute for Medical Research and Occupational Health, Department for Radiation Protection Ksaverska cesta 2, HR-41001 Zagreb, P.O. Box 291, Croatia

Due to chemical and metabolic similarity to calcium, bone is the critical organ for radioactive isotopes of strontium.

Long term-data on 90Sr activities in bones of some domestic animals (cows, pigs and lambs) are presented. As a refractory component of the radioactive debris originating in the Chernobyl nuclear accident, strontium was not subjected to global dispersion processes, being mainly deposited around the accident site. Therefore, in Croatia the Chernobyl nuclear accident caused only slight increase in the lamb bones, while bones of cows and pigs remained practically unaffected.

Using simple mathematical model, turnover rates and corresponding mean residence times of 90Sr in bones for respective species were estimated.



PP43

MOBILE RADIOLOGICAL LABORATORY - REGULAR EXERCISES AND INTERCOMPARISON MEASUREMENTS

B. Pucelj, M. Korun, R. Martincic, M. Ravnikar

Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia

Mobile radiological laboratory was founded in early eighties when the first nuclear power plant in Slovenia was commissioned. The main aim was to provide skilled manpower and equipment for independent field measurements in case of nuclear or radiological emergency. The main equipment nowadays consists of: a germanium detector mounted in the van for measuring different kinds of samples, in-situ germanium detector, portable monitors for measurement of external radiation, surface contamination with beta and gamma emitters, continuous measuring system for external radiation based on GM tubes which is operational during the voyage, pressurised ionizing chamber coupled with a GPS system to correlate dose-rate measurements with the position of the van, samplers for aerosols and different forms of iodine, sampling and sample preparation equipment, meteorological station and personal protective equipment.

There is a negligible possibility that equipment and teams will operate properly in an emergency without regular training of teams and working with equipment. For these reasons it has been a practice from the very beginning to have several field exercises each year. As a part of the emergency programme the team visits three times a year the nuclear power plant and its surrounding. Several field intercomparison measurements of liquid and atmospheric samples are made with the stationary and mobile laboratory of the nuclear power plant. The team visits fixed sampling points around the power plant that are used for a regular monitoring programme and are also planned to present the backbone of the offsite emergency control system. All the equipment is tested in field conditions.

Besides there are other occasions to get more experience - the team has regularly participated in intercomparison field exercises in neighbouring countries and has also been involved in field measurements in suspected and true cases of radiological emergencies.



PP44

MONITORING OF RADIOACTIVE RELEASES AND ENVIRONMENTAL IMPACT OF PAKS NPP

G. Volent, I. Barnabas and E. Viragh

Radiation Protection Department, Paks NPP, 7031 Paks, P.O.B. 71, Hungary

The Paks Nuclear Power Plant runs with four Soviet-designed VVER-440 type reactors, each of 440 MWe capacity. The first unit went into operation in 1983, the fourth reactor unit in 1987. Like many industrial activities, the operation of nuclear power plants entails the production of effluents which are released into the environment.

The health authority has limited the maximum radioactivity discharges to the environment in such a way, that no one of the surrounding population could accumulate more than 250 uSv/y effective dose equivalent relating to 1 GWe capacity. The corresponding limits for airborne and liquid effluents are 167 uSv/y and 83 uSv/y effective dose equivalent, respectively. According to these regulations derived limits are established for gaseous and liquid discharges.

At Paks NPP the monitoring of radioactive releases and environmental presence of radioactive material are performed by telemetric systems and analysis samples taken from emissions and environment. The sensitivity requirements of these measuring methods need to be met the derived limits and potential activity concentration in different environmental media.

The introduction of above mentioned monitoring programme and of the recent results are the subject of our poster paper.



PP45

DETERMINATION OF RADIOSTRONTIUM AND ACTINIDES IN SOME ENVIRONMENTAL SAMPLES OF ALBANIA

E. Gjeci, Xh. Myteberi

Institute of Nuclear Physics, Tirana, Albania

A modest activity of environmental radioactivity monitoring started at INP nearby 1980. Especially, during and immediately after the Chernobyl accident some efforts on gross alpha - beta contamination of air, fallout, milk, vegetables, soil and waters, as well as emitters determination were performed. Taking into account the fact Sr-90 is one of the more hazardous fission products, two different radiochemical separation methods are used for some samples like soil, fresh and powder milk as well as sediments. Sr-90 activity concentration is determined by LSC of the dissolved precipitate,also by gross beta low-level counting method. The results and dynamics of Sr-90 in milk during 1986-1987 are presented. Some nowadays measurements are given, too.

Regarding actinides determination in Albanian soil and sediments, several radiochemical manipulation were necessary. The choice of a particular method was the object of some criteria, like its selectivity and separation efficiency. A brief description of the necessary steps for actinides separation method is given, including the dissolution of ashed sample with mineral acids, the selective anion exchange chromatography method for Pu, Am, U, Th separation from Am of U by liquid-liquid extraction with conc. TBP and finally the preparation of thin sources by rare earth fluoride cooprecipitation using membrane filters.

The measurements of actinides by a Canberra alpha-spectrometric system supplied with a solid state (PIPS) detector are presented. The results of our lab. and that of IAEA (Seibersdorf) are reported.

References:

  1. P.Skende, Xh.Myteberi et al. Proceed. of 1st BPU Conference, Thessaloniki, Greece, (1991),
  2. M.Kedhi, Journ. of Radioanal. and Nucl.Chem. 146/2/(1991),
  3. L.Qafmolla,Xh.Myteberi, Proceed. of General Conference of BPU, Izmir, Turkey (1994),
  4. J.J.LaRosa et.al. J.Environ.Radioactivity 17 ,183-209, (1992),
  5. N. Vajda et.al. J.Radioanal. Art.Vol 162 No2, 307-323, (1992) [6] Xh. Myteberi, E.Gjeci Reports of INP, Tirana (1994).



PP46

FIELD MEASUREMENTS ON HIGH ALTITUDE ALPINE AREAS OF AUSTRIA

A. Andrasi 1, H. Lettner 2, E. Lovranich 3, F. Steger 3, J. Urban 1, E. Urbanich 3 and P. Zombori 1

1 KFKI Atomic Energy Research Institute, Budapest, Hungary
2 University of Salzburg, Austria
3 Austrian Research Centre Seibersdorf, Austria

Connecting to an international intercomparison exercise of mobile laboratories organized in Gera (FRG) in 1993 a satellite action was organized by the three teams to investigate the radiological situation in some high altitude Alpine regions of Salzburg province. The places were selected for the high natural (Ra) and artificial fallout (Cs-137) activity concentration detected earlier in this region. In situ gamma spectrometric and dose rate measurements were performed in three places of different site characteristics: (a) on an undisturbed grassy meadow in Salzburg, on Alpine meadows (b) near Badgastein (Nassfeld) and (c) in Obertauern. These measurements were the basis for the site selection of a larger scale international intercomparison exercise in 1994.

The measurements confirmed the high fallout radionuclide concentration of Chernobyl origin and gave an indication of very different depth distribution characteristics in the soil. A new method of in situ gamma spectrometry with collimated detector arrangement was tested and compared to the traditional uncollimated wide area monitoring method. In the course of the exercise the recently established on-route monitoring system was used. With this investigation interesting fluctuations in the environmental radiation level due to natural radioactivity was detected.

The results of the measurements obtained during the field exercise will be presented in the paper.



PP47

ENVIRONMENTAL MONITORING OF 137CS IN THE VARDAR RIVER CATCHMENT AREA

T. Anovski 1, L. Cvetanovska-Nastevska 2, N. Jovanovski 2

1 Faculty of Technology and Metalurgy, Skopje, Macedonia
2 Center for Application of Radioisotopes in Science and Industry, P.O.Box 274, 91000 Skopje, Macedonia

Distribution of 137Cs, as one of the most important anthropogenic radioactive pollutant on the environment, in various samples within the Vardar river catchment area has been determined.

By application of radioecological. model on effective dose equivalent for different transfer media and exposure pathways as a contribution of 137Cs to the total exposure of a man were calculated.



PP48

ENVIRONMENTAL RADIOACTIVITY AROUND THE FORMER COAL MINE

M.Krizman, B.Pucelj, M.Korun, D.Konda, J.Smrke

Jozef Stefan Institute, Jamova 39, SI-61111 Ljubljana, Slovenia

Soon after World War II it was recognized that brown coals from Lower Carniola (coal mines in Kocevje, Kanizarica, Vremski Britof) contain quite high amounts of uranium, up to ten times more than other coals in Slovenia. Enterprises were obliged to collect coal ash; it was intended for further processing and yellow cake production, but due to an insufficient content of uranium these plans were never realized. In Kocevje, the coal mine was in operation from 1803 and ceased production in 1972. Huge amounts of coal mining wastes and coal ash were freely disposed of on an area (1.25 km2) between the town of Kocevje and the nearby village of Salka vas. Excavated underground shafts collapsed and a lake with an area of 0.25 km2 appeared in the vicinity of the town.

A pilot research study was performed recently concerning the levels of radioactivity in the mine environment to acertain the possible impact of the former mining activities on the surroundings. A comprehensive programme of sampling and radiation measurements covered the following items: gamma dose-rate measurements on the coal and ash tailings deposit and outside the area, analysis of deposited materials, radon and radon daughter measurements outdoors and indoors, and radioactivity of the lake water.

Results showed that coal samples and mixtures with ash, coal and soil contain high quantities of uranium and radium. Great variations in contents of natural radionuclides (U-nat, 226Ra) were found, mainly in the range of 400-1200 Bq/kg, but in some places even more than 4000 Bq/kg. Radioactivity in the disposal terrain is not uniformly distributed; in some parts of the depository gamma dose-rates up to 0.3-0.4 uGy/h were measured. Mainly, values of 0.20-0.25 uGy/h were found over the total area. Radon in dwellings was also measured: winter daily radon concentrations in houses, built on or near the affected area, reach up to 2600 Bq/m3 with an average of 200 Bq/m3 in living rooms, while in cellars concentrations in one case reached 3150 Bq/m3. Most of these houses are made of local clay bricks, so indoor gamma dose rates were expected to be enhanced; we found values mostly around 0.15 Gy/h. Due to leaching of excavated materials by precipitation, the radioactivity of lake water (and also seepage water) is evidently higher than in other surface waters, i.e. at minimum by an order of magnitude: 226Ra 30 Bq/m3, 238U 160 Bq/m3. Some measurements are still in progress.

The town of Kocevje is situated in a totally closed circular valley. In the period of strong temperature inversions we measured relative high radon and radon daughter concentrations: for radon a daily average about 80 Bq/m3 with early morning maxima even up to 150 Bq/m3. These are surprisingly high figures when compared to simultaneously measured values in the region of the uranium mine area around the Zirovski vrh. In spite of a large U mine waste deposits and tailings pile, which represent high emission sources of radon, the concentrations of outdoor radon in the nearby surroundings of the uranium mine never reach these values. Uranium contents in soil in the Kocevje region far exceed the national average level. This feature, together with millions of tonnes of waste coal tailings and ash, are obviously the reason for the highest occurrence of outdoor radon. The map of indoor radon in Slovenia also confirms this finding: the Kocevje community is categorized among radon prone areas with an average annual indoor concentration of radon being 160 Bq/m3.



PP49

TERRITORIAL NETWORK OF TLD IN CZECH REPUBLIC

D.Kroutilikova, Z.Prouza, L.Hobzova

Centre of Radiation Hygiene, National Institute of Public Health, Prague, Czech Republic

The territorial network of the thermoluminescence dosimeters (TLD) is one of the most important components of the Czech Radiation Monitoring Network (CRMN). Recently, a modernization of the instrument equipment and the dosimetry has been realizing. From 1996 the CRMN will use the TLD system HARSHAW 4000 along with the type 8807 environmental dosimeter. The poster summarizes both the hitherto experiences of the use of the TLD in CRMN and results obtained at a testing of the new system and the new dosimeters.


PP50

STUDY ON DETERMINATION OF PLUTONIUM ISOTOPES IN SOILS FROM LUBLIN REGION (POLAND)

A. Komosa

Department of Radiochemistry and Colloid Chemistry, Maria Curie-Sklodowska University, Pl.M.C.Sk odowskiej 3, 20-031 Lublin, Poland

Up till now the region of Lublin (eastern part of Poland) have not been studied as concerns a contamination with the alpha-emitting transuranium isotopes. This is why we have undertaken a study in this field. We have developed the methods for plutonium and americium separation from environmental matrices and the alpha spectrometry measurements as a result of a cooperation with J.Stefan Institute in Ljubljana (Slovenia).

The analytical quality of the method of plutonium isotopes determination was verified by analyzing the IAEA reference material: Soil-6. Using a Students's t-test we found that a difference between Pu-239,240 contents obtained and a certified value is statistically insignificant.

For plutonium radiation measurements we use the Canberra's alpha spectrometer equipped with partially depleted PIPS detector of 20 keV FWHM resolution, and efficiency of 46.5%.

We determined the plutonium isotopes contents in the samples of upper layers of different soils collected in Lublin region. It was found that the amount of Pu-239,240 in all samples ranged from 0.074 to 0.337 Bq per kg dry weight of soil, and Pu-238 from MDA to 0.026 Bq/kg. The ratio of Pu-238/Pu-239,240 suggested rather a fallout origination of plutonium isotopes determined.

The minimum detectable amount (MDA) of plutonium was calculated to be 2 - 15 mBq/kg of soil depending on radiochemical yield (as found with Pu-242 tracer) and a time of measurement.



PP51

STUDIES OF THE PRESENCE OF GAMMA EMITTERS IN THE NATURAL ENVIRONMENT OF EASTERN POLAND

S. Chibowski, J. Szczypa, J. Zygmunt

Department of Radiochemistry and Colloid Chemistry, Faculty of Chemistry, Maria Curie Sk odowska University, 20-031 Lublin, Poland

The results of the measurements of the radioactivity level of soil and grass samples of Eastern Poland as well as of the ground layer of the atmosphere are presented. Natural and artificial gamma emitters are distinguished in the presentation. The total activity of soil samples ranges from 200 to 1200 Bq/kg with 55-70% contribution of potassium 40. The rest is due to the presence of the following natural: Ra-226, Bi-214, Pb-214, Th-234, Ac-228, Bi-212, Pb-212, Ra-224 and Th-228 and artificial: Cs-137 and Cs-134 radionuclides.

From the ratio of activities of Cs-134 and Cs-137 just after the Chernobyl accident, the contribution of after-Chernobyl Cs-137 and that from the global fall out to the total Cs-137 activity can be calculated in particular segments of soil profiles. These data may be used to calculate the vertical migration rates in various types of soil. In 1994 the after-Chernobyl radiocesium was found in the uppermost soil layer down to about 10 cm. Its average contribution to the total contamination of the uppermost 5 cm layer with cesium averaged 77%.

The total activity of grass in the studied area ranged from 15 to 1375 Bq/kg of dry matter. The activity of radiocesium in grass in the studied area ranged from 1 to 172 Bq/kg of dry matter and it depends on the type of soil and on the contents of potassium in the soil. The calculated transfer factors (TF) of Cs-137 from soil to grass range from 0.03 to 21 and in most cases they decrease when TF of K-40 increases.

The radioactivity of the ground layer of the atmosphere was as low as 1.2 to 3.4 mBq/m3.

The present results suggest that there was no substantial radioactive fallout in Central-Eastern Poland over the last year.



PP52

NATURAL AND ARTIFICIAL RADIONUCLIDES IN LICHENS AS AIR POLLUTION MONITORS

Z. Jeran 1, R. Jacimovic 1, Franc Batic 2, A. Prosenc 1

1 Jozef Stefan Institute, Jamova 39, 61111 Ljubljana, Slovenia
2 Biotechnical Faculty, Department of Agronomy, Jamnikarjeva 101, 61111 Ljubljana, Slovenia

Epiphytic lichens, symbiotic organisms composed of an algae and fungus, are efficient accumulators of many elements, particularly heavy metals and radionuclides that are released into the atmosphere because of natural or human activities. In 1992 a national biomonitoring programme was initiated covering the whole territory of Slovenia to measure the levels of some natural (210Pb, 40K, U, Th) and artificial (137Cs, 134Cs) radionuclides in the epiphytic lichen Hypogymnia physodes L. (Nyl.) as to obtain information on their levels in our environment.

The epiphytic lichen Hypogymnia physodes L. (Nyl.) was collected at 86 sampling points of the 16 x 16 km bioindication grid of Slovenia and the levels of 210Pb, 40K, 134,137Cs were determined by direct counting of dry samples using gamma spectrometry. U and Th levels were determined by the k0-standardisation method of Instrumental neutron activation analysis.

The results are presented as geographical isocontours of radionuclide activity on a national scale. The geographical distribution of radionuclides obtained from lichen data were divided into 7 classes according to percentile values (10, 30, 50, 70, 90 and 95 %) and were mapped using the Surfer programme.

Each of the radionuclides analysed has its own geographical distribution pattern as a consequence of its origin. 210Pb is the long lived radionuclide produced in the atmosphere by radioactive decay of its gaseous parent 222Rn, 40K, U and Th are natural radionuclides contained in the lithosphere, but 137+134Cs were released to the atmosphere during the Chernobyl accident and in atmospheric nuclear tests.

The mean value of 210Pb was about 600 mBq g-1, with the highest activity levels up to 1900 mBq g-1 in lichens collected in the southern - Dinaric region of Slovenia.

40K levels were in the range between 65 - 290 mBq g-1. Elevated levels were found in NW and W parts and at some locations in the east of Slovenia. Also the U and Th levels in lichens were low as expected, with mean value of 0.12 and 0.29 g g-1, respectively. The highest activity of both Cs-isotopes was found in samples from the north and north-west parts of Slovenia, which are known to have received the highest amounts of precipitation during the period following the Chernobyl accident.



PP53

ENVIRONMENTAL RADIOACTIVITY DUE TO FLY-ASH DISPOSAL - RESULTS OF A MONITORING PROGRAMME

M.Krizman * and L.Mljac **

* Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia
** ERICo, Velenje, Slovenia

The o tanj coal-fired power plant (750 MWel) has been in operation for more than 20 years and currently produces almost a million tonnes of coal ash per year. Fly ash with a U content of 25 mg/kg is transported as a slurry and disposed firstly into lake water and later into wet ponds. The whole area including the disposal site lies on sinking terrain due to coal mining and excavation, and several lakes were created after flooding of the land. The largest of them is located just on the edge of the fly ash deposit, so water has direct contact with the deposited ash. The size of the landfill area is about 50 ha, including the wet ponds and dry part of the disposal site, partly covered with a soil layer and recultivated.

Radioactive materials released into the environment are dispersed and transferred through various environmental pathways, leading to external and internal radiation exposure. A short term surveillance programme was conducted to investigate these routes.

Results showed enhanced gamma radiation: dose-rate levels are significantly higher mainly within the area of the uncovered deposited material. Airborne radioactivity also originates from dry uncovered surfaces: the important pathways are inhalation of dust particles with long-lived radioactivity, and inhalation of radon with its short-lived progeny. Periodic high concentrations of air particulates due to wind erosion of bare areas, were observed even at moderately distant locations. Superficial radioactive contamination of vegetables and grass was also taken into account and measurements are still in progress. Surprisingly, the average concentrations of radon and its daughters over the landfill were in very similar to those in its nearby vicinity. The attention at this point is now focused on short term measurements, preferably in very stable weather conditions.

Leaching of radionuclides with lake and rain water and pile drainage water are the main sources of radioactive contamination of the lake, its outflowing waters and sediments.

The high alkalinity of lake water due to the presence of fly ash (the pH is nearly 11) strongly influences the solubility and therefore the radionuclide concentrations: a very low concentration of uranium was measured while radium (226Ra) is present in concentrations an order of magnitude higher than in other uncontaminated waters. River sediments also showed increased river bed radioactivity even at longer distances from the discharge points.

As far as we know, a similar surveillance programme on fly-ash disposal has not been performed elsewhere; the main conclusion of some previous investigations, covering only some of the pathways, was the absence of any radiological impact. Based on our results, an extended programme will be carried out next year to ensure a more complex evaluation of the environmental impact. The programme will also include radioactivity measurements of local precipitation, continuous measurements of radon and its daughters, and extended measurements of radon exhalation rates from various materials. It will ensure the present state of radioactive contamination on the site and its surrounding is precisely defined and later, to assess possible positive effects of remediation measures and restoration of the site.



PP54

RADIATION WARNING SYSTEM IN SLOVENIA (ROSS)

S. Arh

Slovenian Nuclear Safety Administration, Slovenia

The primary task of the system is to detect any incidents involving radioactivity as fast as possible, to initiate appropriate measures, and to give warning to the population immediately.

The system will consist of 30 gamma dose rate stations and 2 alpha and beta aerosol monitors connected to the central computer. Meteorological data will be also collected.

A radiological network of four stations around NPP Krsko already works. In 1995 it will be supplemented with 9 new gamma monitors on different places. Data are collected automatically on every half an hour.

10 independent gamma monitors already work on meteorological stations. Data are manually collected once a day by phone call to the sites. Automatic connection to the centre is planned via the public switched telephone network. Gamma monitors are MFM-202, made in Slovenia by Institute "Jozef Stefan". Alnor Area Radiation monitoring System AAM-95 is also tested.



PP55

137Cs IN NORTHEREN ADRIATIC SEDIMENTS

D. Barisic, S. Lulic, A. Vertacnik, N. Vdovic, M. Jurasic

1 Center of Marine Research - Department Zagreb, "Rudzer Boskovic" Institute, Bijenicka 54, Zagreb, Croatia
2 Department of Geology, Faculty of Natural Sciences, University of Zagreb, Croatia

The activity of 137Cs in shallow northern Adriatic sediments was obtained on the basis of the measurement results from 21 sediment box cores, sampled during the ASCOP 16 cruise in the summer 1990. 137Cs was determined in surface sediments (0 to 3 cm) and 12 to 15 cm deep sediment. It was found that the lowest caesium concentrations correspond to sands which are spread along the Croatian coast. Parallel to the Italian coast, 137Cs concentrations in pelites are the highest. It seems that the influence of Po River is significant for 137Cs activities in recent marine sediments along Italian coast south of Po River delta. Significantly higher 137Cs activities in 0 to 3 cm sediment layer can be attributed to the deposition caused by Chernobyl accident.


PP56

A LONG-TERM STUDY OF CAESIUM TRANSPORT IN A RIVER OF THE ITALIAN ALPINE REGION AFTER THE CHERNOBYL RELEASE

P. Spezzano, S. Bortoluzzi, R. Giacomelli, L. Massironi

ENEA - Dipartimento Ambiente, AMB-ICR-TER, CR Saluggia, Italy

Concentrations of 137Cs in water were monitored after the Chernobyl accident from January 1987 to December 1991 in the Dora Baltea river (northwest Italy), a river characterized by a catchment area located in the Italian Alpine region. The Dora Baltea river (160 km in length and average flow rate of 110 m3/s) originates from the massif of Mont Blanc (4810 m of altitude) and flows in the Po river. Its basin, of 4322 km2, collects most of the waters from the western alpine mountains in a region which is the most intensely covered with glaciers (about 190 km2) of the Italian side of the Alps.

A strong seasonal variation of water 137Cs concentrations was observed, with elevated concentrations in summer and lower concentrations during all the other seasons. Increased water concentrations in summer were attributed to caesium deposition and accumulation on snow-covered surfaces in winter and then released in summer during ice and snow melting as a consequence of the seasonal increase of temperature. An attempt of relating the observed cyclical variations with estimated transfer rates from the catchment has also been performed.



SESSION IV:
NUCLEAR INSTRUMENTATION AND DOSIMETRY


OP31

CHARACTERIZATION OF TL DOSIMETERS FOR DETERMINATION OF THE GAMMA COMPONENT IN A MIXED n+ RADIATION FIELD

M. Ranogajec-Komor, S. Miljanic, M. Osvay *, S. Ferek, I. Dvornik

Rudzer Boskovic Institute, 41000 Zagreb, P.O.B. 1016, Croatia
* Institute for Isotopes, 1526 Budapest, P.O.B. 77, Hungary

Detailed measurements of sensitivity, linearity, supralinearity and fading of the TLD-100, TLD-700, CaF2:Mn and Al2O3:Mg, Y detectors with various encapsulations were carried out to asses the suitability of these detectors for measuring total gamma dose in a mixed n+gamma irradiation field during the International Intercomparison of the Criticality Dosimetry Systems organized by the Commission of European Communities at SILENE Reactor in Valduc, 1993.

After mixed field irradiation, some detectors were read at Valduc, others at the Ru er Bo kovi Institute (RBI). The readings have shown the agreement between the Valduc and RBI gamma field calibrations. After readout the recalibration of the response to gamma rays and accurate determination of fading kinetics was performed. No change of sensitivity after neutron irradiation could be observed with TLD-700 and CaF2:Mn detectors. The reproducibility of Al2O3:Mg, Y detectors deteriorated somewhat, with no systematic change of sensitivity. The sensitivity of TLD-100 detectors changed after neutron irradiation.



OP32

CALCULATED ALPHA COUNTING EFFICIENCY OF A SAMPLE/DETECTOR GEOMETRY FOR AMBIENT RADON PROGENY MEASUREMENT

R. Rolle, H. Lettner, W. Hofmann, R. Winkler

Institute of Physics and BIophysics, University of Salzburg, Austria

Alpha measuring instruments for ambient radon progeny are usually calibrated by comparison measurements in an official radon chamber. An alternative, or additional way of calibration, is the calculation of the efficiency from specifications of the measuring geometry.

The alpha detection efficiency is determined by the effective solid angle and by the alpha energy absorption in the various sections of the sample/detector geometry. For most commercial instruments, with concentric sample and detector, absorption along the longest path, i.e. diagonally across the measuring geometry, is sufficiently low for an alpha particle still to produce a detector signal above a threshold. In that case only the effective solid angle needs to be calculated for the gross alpha counting efficiency. For point sources the solid angle subtended by the detector can be calculated, and the effective solid angle is obtained by averaging for source elements over the whole source. In the more general case of spectrometric efficiency the effective solid angle needs to be evaluated for specific intervals of residual energy of alpha particles that reach the detector.

In a preliminary study using a certified alpha source, calculated and measured efficiencies showed good agreement under varied measuring geometries. The use of the calculation method of calibration could complement, or even to some extent replace the more costly radon chamber calibration of radon progeny instruments and should assist in better quality assurance in the assessment of public radiation exposure.



OP33

MEASUREMENT OF DISSOLVED RADON AND RADIUM CONTENT OF WATER SAMPLES BY TRACK ETCH TECHNIQUE

J. Hakl 1, I. Hunyadi 1, I. Csige 1, J. Somlai 2, G. Faludi 2, K. Varga 3

1 Institute of Nuclear Research of the Hungarian Academy of Sciences, H-4001 Debrecen, POB 51, Hungary
2 Department of Radiochemistry, University of Veszprem, H-8200 Veszprem, Egyetem ut 10, Hungary
3 Bessenyei György Teacher's Training College, H-4401 Nyiregyhaza, POB 166, Hungary

We have developed a method to determine dissolved radon and radium content of water samples using track etch type radon monitors. In two measurements the radon exposures in a freshly sealed and in a degassed water sample are determined. From the measured exposures the radon and radium content of fresh water is calculated. The method can be applied as well for in situ integrating measurement of total radon content of natural waters. The results of theoretical and experimental calibrations will be presented together with some results of field test studies.

We found that the method allows a cheap and simultaneous examination of a large number of samples.



OP34

TSEE CHARACTERISTICS OF LiF:M,C,P DETECTORS

G. Uchrin

Institute of Isotopes of the Hungarian Academy of Sciences, H-1525 Budapest, P.O.Box 77, Hungary

LiF:M,C,P detectors are highly sensitive to their heat treatment, annealing above 240 deg C usually destroys their thermoluminescence, TL, properties. Thermally stimulated exoelectron emission, TSEE, glow curve exhibits peaks much higher than the main TL dosimetric peak. It was revealed that the TSEE glow curve did not change significantly when the detectors were red out up to 500 deg C and this readout was repeated more than ten times. LiF:M,C,P detectors from Poland, Krakow, INF type MCPN-S and from China, Model GR-200, have been investigated using a multi-needle type GM detector based TSEE reader, developed at Fontenay-aux-Roses, France. The main TSEE parameters of these detectors such as glow curve, sensitivity, dose response, fading, minimum detectable dose, energy dependence of beta dose measurement, etc. are given and compared with other LiF,Mg,Ti detectors.


OP35

EQUIVALENT DOSE MEASUREMENTS IN AIRCRAFTS WITH TLD S UNDER CONSIDERATION OF THE PEAK HEIGHT RATIO

M.Noll, W.Schöner *, M.Fugger *, N.Vana *, H. Brandl **

Institute for Space Dosimetry, A-1190 Vienna, Döblinger Hauptstrae 7, Austria
* Atominstitute of the Austrian Universities, A-1020 Vienna, Schüttelstrae 115, Austria
** Institute of the German Airforce, D-82242 Fürstenfeldbruck, Germany

For dose measurements in unknown mixed (n, )-fields in aircrafts thermoluminescence dosemeters were used embedded in poystyrol or polyethylen of varying thickness (25 cm diameter spheres, 2 cm polystyrol, 2 mm polystyrol). Beside the determination of the absorbed dose the evaluation of the linear energy transfer (LET) with the method of the peak height ratio was determined. Furthermore the peak height ratio makes the determination of the different fractions induced by gammas, thermal neutrons or other high-LET radiation depending on the poystyrol thickness possible.

For evaluation of the fraction of thermalized neutrons and fast neutrons (including protons and other charged particles) of the equivalent dose the neutron energy dependence of the TL-response was calibrated using TLDs embedded in polyethylen spheres (diameter 25 cm) in a special arrangement. The calibration was performed with several neutron sources (thermal, Pu-Be, Am-Be and 14 MeV neutrons).

The results show that with the applied method information of the fraction of the different kind of radiation depending on the geometry can be obtained. Additional measurements with active systems were performed and the results compared.



OP36

QUANTITATIVE DETERMINATION OF THE TRANSURAN ISOTOPES FROM EVAPORATING RESIDUE AND PURIFIED WATER DISCHARGES OF NUCLEAR POWER PLANT PAKS

* I. Gresits, * S. Tölgyesi, * J. Solymosi, * L. Gy. Nagy, ** T. Past, ** L. Szabo, *** P. Ormai

* Technical University Budapest, Department of Physical Chemistry, H-1521, Budapest, Hungary
** Ist Dept. of Medicine, Medical University of Pecs H-7643 Pecs, P.O. Box: 99, Hungary
*** NPP Paks, 7031, Paks, Pf.71., Hungary

New analytical procedures on the alpha-emitting isotopes of evaporating tailings and proposed purified water discharges were developed. During sample treatment of the evaporating tailings the samples were decomposed by oxidation after removing of the big bulk of boric acid. Samples of the purified water discharges were concentrated by an unusual process based on a microwave technology.

Thin sample layer for the alpha spectroscopy was prepared on a new way in a cathode potential regulated electrodeposition cell to increase selectivity. The activity-concentration values were calculated in a usual way know from the literature. The usefulness of process are demonstrated on authentic sample spectra.



OP37

SELECTIVE INSTRUMENTAL MONITORING OF RADIOIODINES IN NPP PRIMARY COOLANT

J. Simon, E. Erdos, J. Soos, T. Pinter *, P. Zagyvai **, A. Gujgiczer, R. Chobola, J. Solymosi, L. Gy. Nagy

Technical University Budapest, Department of Physical Chemistry, H-1521, Budapest, Hungary
** Technical University Budapest, Institute of Nuclear Technics, H-1521, Budapest, Hungary
* NPP Paks, 7031, Paks, Pf.71, Hungary

Continuous analysis of radioiodines in pressurised water type nuclear power plant primary coolant produces information about the state of the fuel element cladding. An immediate detection of cladding failure is important in reactor safety.

Direct measurement of the coolant is disturbed by it's high matrix activity, therefore radioiodines have to be separated.

A method has been developed to select radioiodines by chemical separation. Iodine selectivity of the method was determined and proved. Neither ionic or non-ionic nor gaseous components were found in the selected sample.

On the basis of this method a computerised apparatus has been built and tested at the Hungarian power plant at Paks city. Radioactive concentration of all of the five radioiodine isotopes are continuously monitored selectively and results are produced in every 15 minutes.

Characteristics of the apparatus:

- high selectivity of radioiodine analysis
- for gamma-spectrometry a simple NaI(Tl) scintillation detector is applied
- simple and not expensive accessories and materials are used
- there is no radioactivity accumulation in the system during a long period of operation
- automatic operation without the need of human control for several weeks
- apparatus as an industrial equipment can be placed on line primary coolant sampling.

Apparatus is advised to be placed in pressurised water type nuclear power plants especially in Eastern Europe, Russia, Ukraine etc.



OP38

INTELLIGENT NUCLEAR SPECTROMETER

Z. Illes, A. Gujgiczer, L. Simoncsics, O. Zsille, G. Plachtovics, J. Solymosi

Technical University Budapest, Department of Physical Chemistry, H-1521, Budapest, Hungary

This small device makes the nowadays just wide-spread personal computers (IBM PC/AT compatible) suitable to measuring gamma-spectrum by using most of the NaI(Tl) scintillation probes.

The main purpose of the development was making a low-cost device, that employs the existing old-type scintillation probes in multichannel analyzer, taking out the simple multiscalers.

The device based on an 8-bit microcontroller. This one deals with the data collection and the communication towards the PC. The signals coming from the scintillation probe are received by a 256-channel Wilkinson-type A/D converter (programmable amplification). The also programmable output high voltage to the photomultiplier has an excellent dc stability ( 800-1200 V +- 0.1%).

The communication towards the PC is through the very popular RS-232C interface.

The device can run on battery or on ac power supply, suitable on in-situ measurement too.

The handling program is running on the PC under the Microsoft Windows v3.1 environment. Using the possibilities of the operation system (Dynamic Data Exchange = DDE) the measured data can also be processed with other popular software (e.g.: MS-Excel, Lotus 1-2-3 etc.).

The base-software contains:

- setting the amplify and the high voltage
- count rate monitoring
- calibration: energy, efficiency, FWHM
- peak search
- smoothing (5, 7, 9 points)
- documentation
- some built-in standard measuring method



OP39

A PROCEDURE FOR THE CONTINUOUS CONTROL OF THE RETENTION PROPERTIES OF GAS ADSORBER SYSTEMS

A. Vincze *, G. Volent **, J. Solymosi

* Technical University Budapest, Department of Physical Chemistry, H-1521, Budapest, Hungary
** NPP Paks, 7031, Paks, Pf.71, Hungary

The retention properties of the charcoal based radioactive gas adsorber systems are key parameters as far as the continuous release of fission product gases at NPP Paks is concerned. The retention of the radioactive noble gases takes place on the charcoal adsorber by dynamic adsorption, meanwhile their activity decrease according to their half-life-times.

For the optimal operation of the adsorber units the on-line control and analysis of the retention properties would be required. Therefore a procedure has been developed for the determination of the retention times and the dynamic adsorption coefficients for the specific noble gas isotopes. The method is based on the continuous analysis of the in- and out-flow of the adsorber system by gamma- ray spectroscopy using semiconductor detectors.

After the successful laboratory test, the procedure was installed and the retention properties of a charcoal based radioactive gas adsorber system were determined.

For the evaluation of the data, a theoretical model was developed, which was used for the calculation of the dynamic retention coefficients of the noble gas isotopes.

The brief introduction of the procedure and some relevant results are the subject of the presentation.



OP40

IN-SITU GAMMASPECTROMETRY INTERCOMPARISON EXERCISE IN SALZBURG / AUSTRIA

F. Steger 1, H. Lettner 2, A. Andrasi 3 and E. Lovranich 1

1 Austrian Research Center Seibersdorf, Department Radiation Protection, Austria
2 Institute of Physics and Biophysics, University of Salzburg, Austria
3 Health Physics Department, KFKI Budapest, Hungary

In-situ gammaspectromety has become a useful method to assess the nuclide concentration of artificial and natural gamma-emitters in the soil. For the quality assurance of the measurements periodically intercomparison exercises are essential. To meet this requirement exercises were organized in different European countries since 1989. The last exercise in September 1994 was organized in Salzburg / Austria. The participation of approx. 30 measurement teams from all over Europe emphasizes the importance of the intercomparison. Salzburg was selected because the Province of Salzburg / Austria was among the heaviest contaminated region outside the former USSR by the Chernobyl fallout. Two different typical sites were selected for the measurements: Site 1 was inside the urban area of Salzburg on intensively used agricultural land which had not been disturbed since the fallout. This site is representative for intensively used agricultural regions in the Province of Salzburg. Site 2 was in the mountainous region of the Tauern on elevated altitude of approx. 1700 m. This site represents the soil and contamination conditions of the Alpine region. Both sites differ significantly in terms of different soil distribution that is crucial for the evaluation of the gamma spectra. The participants use different approaches for the evaluation of the gamma spectra in terms of consideration the depth distribution. The results are presented.


OP41

THE IMPORTANCE OF LOCALISATION WITHIN 131J-RETENTION MEASUREMENTS

G. Greifeneder 1, H. Aiginger 1, F. Steger 2, J. Flores 3

1 Atominstitute of the Austrian Universities, A-1020 Vienna, Austria
2 Austrian Research Center Seibersdorf, A-2444 Seibersdorf, Austria
3 Department of Nuclear Medicine, University of Vienna, A-1090 Vienna, Austria

A widely used method to investigate thyroid carcinomas, but also disorders of the thyroid function is the measurement of the 131J-retention using a whole body counter. Normally just the retention of oral administered radioiodine is controlled. We developed a method to analyze the distribution of 131J beside the retention in the human body which provides much better information on human metabolism.

To demonstrate the power of this high sensitive method we investigated patients with total thyroid ectomie. To ensure the absence of new metastasis oral dosis with 20 uCi has been provided. One hour and 72 hours later profile scan measurements with a whole body counter using a special detector configuration have been done. Looking just at the retention values the possible presence of thyroid tissue cannot be excluded of certainty but regarding the spatial resolution in addition a decision between localisation and dislocalisation is possible. Therefore it can be decided about the physiological or pathological meaning of these retention values.



OP42

QUALITY ASSURANCE OF ACTIVITY MEASUREMENT IN RADIATION MONITORING NETWORK OF CZECH REPUBLIC

I.Malatova, D.Drabova

Centre of Radiation Hygiene, National Institute of Public Health, Prague, Czech Republic

Centre of Radiation Hygiene of NIPH is in charge of running Radiation Monitoring Network of Czech Republic (RMN). One from main task of the RMN is to follow activity of artificial radionuclides in different components of environment, in food chain and in biological samples from which internal contamination of people could be estimated. Results from whole-body counting are included, too. Altogether 12 laboratories, equipped by semiconductor gamma spectrometry regularly supply the measured data about the radionuclide activity concentration in different samples.

To ensure compliance of the measurement from all laboratories, interlaboratory comparisons are organized by the Centre of Radiation Hygiene NIPH at least once in a year. For the aim of the intercomparison exercises, different reference material with unknown mixture of radionuclides is usually supplied to individual laboratories of RMN. As one of their important task is to determine radionuclide activity in the case of any radiation accident as quick as possible, intercomparison exercise was aimed a.o. on the quick response and on the determination of radionuclides activity in sample of non-standard measuring geometry. Laboratory of gamma-spectrometry of the CRH NIPH, who organizes these intercomparisons, participates regularly in international intercomparisons, including intercomparisons of whole body counting.



PP57

DETERMINATION OF THE SELF-ABSORPTION IN ENVIROMENTAL SAMPLES OF MARINELLI-GEOMETRY AND HPGE-DETECTORS USING MONTE-CARLO-SIMULATIONS

H. Russold, Hj. Müller, H. Rabitsch, W. Ninaus

Abteilung für Strahlenphysik, Institut für Theoretische Physik, Technische Universität Graz, Petersgasse 16, A-8010 Graz, Austia

Measuring smallest activities as required in environmental monitoring demands high efficiencies and large sample volumes. Both are well accomplished by a Marinelli-beaker-geometry but they are affected by the self-absorption.

In gamma-spectroscopy the self-absorption-coefficients are very important if the mean free paths of the photons are different in calibration- and sample-materials due to other chemical compositions or/and different densities.

It is the purpose of this study to find an analytical term for self-absorption for Marinelli-geometry by fitting results of Monte-Carlo-calculations. This term is required to cover the desired energy range as well as arbitrary chemical compositions and densities.

The numerical simulations of self-absorption-coefficients for Marinelli-geometry make use of the Monte-Carlo-transport-code EGS4 for photons and electrons. Calculations are made for photon energies in the range from 20 keV up to 2 MeV for HPGe-coaxial-detectors. We consider environmental samples with densities between 0.1 g/ccm and 2.0 g/ccm. Self-absorption-coefficients are calculated (a) by means of attenuated photon flux and (b) the energy depositions by photons in the detector. Results of both methods are compared with experimental data.

There is a good agreement between the simulated and experimental results.



PP58

CHARACTERISTICS OF X-TEST INSTRUMENT FOR MEDICAL DIAGNOSTIC X-RAY MACHINES

E. Blahak 1, K. Erdelyi 2, S. Pellet 1, L. Szobonya 3

1 "Frederic Joliot Curie" National Research Center for Radiobiology and Radiohygene, H-1775 Budapest, Pf 101., Hungary
2 MicroVacuum Ltd., H- 1 147 Budapest, Kerekgyarto u. 10, Hungary
3 SFW Software Anstalt, H- 1 13 3 Budapest, Kapat u. 44, Hungary

The survey of nuclear radiation exposure of the population showed that about 70-90% of the total dose is originated from the medical diagnostic examination. This high ratio led to the conclusion that optimising the exposure condition plays a very important role in reducing the total radiation dose of the population.

The X-TEST instrument provides a very simple and low cost tool for every-day quality test of the X-ray machines allowing the comparison of the measured dose value to the reference dose levels.

The main characteristics of the X-TEST instrument are small size, portable, rechargeable-accu operated, using Si(Li) detector, automatic reset after exposure. An 8 character LCD display presents the output readings for dose, dose-rate, exposure time and homogeneity factor. The applied small current integrated circuits, microcontroller assure very reliable operation. In addition to the detailed technical characteristics, the results of intercomparison measurements are also going to be demonstrated.



PP59

COMPUTER AIDED NUCLEAR RADIATION MEASUREMENT AND EDUCATIONAL SYSTEM

K. Erdelyi, I. Szendro

MicroVacuum Ltd., H- 1 147 Budapest, Kerekgyarto u. 10, Hungary

Understanding of the basic nature of nuclear radiation plays an important role in education of population for nuclear radiation protection. The developed G-MES computer aided nuclear radiation measurement and educational system is a multipurpose device for education of nuclear physics in secondary and high schools.

In our presentation we will demonstrate the main application fields:

Examination of the statistical nature of the nuclear decay
Examination of the distance dependence of the radiation field
Absorption of the nuclear radiation in different materials
Continuous monitoring of background radiation with alarm

The G-MES system consists of a nuclear radiation monitor, a computer interface, an IBM compatible PC with WINDOWS operation background and the G-MES software.

The G-MES system software utilises all the benefits supplied by the WINDOWS operation. The software can be easily controlled from the MENU items. The measured data are continuously demonstrated in graphics on the display and can be saved and printed. Theoretical and practical information are implemented in HELP file and can be reached without interrupting the measurement. The G-MES system is available in English, German and Hungarian language.



PP60

IN-SITU GAMMA RAY SPECTROMETRY FOR MEASUREMENTS OF ENVIRONMENTAL RADIOACTIVITY

I. Winkelmann, H. Buchröder, Ch. Brummer, M. Thomas

Bundesamt für Strahlenschutz, Waldowallee117, 10318 Berlin, Germany

The method of in-situ gamma ray spectrometry for measurements of environmental radioactivity is described. Results of measurements of natural radionuclides in surface soil by means of in-situ gamma ray spectrometry on some selected characteristic sites in the vicinity of uranium mine facilities in Thuringia and Saxony are presented and compared to those from soil sample analysis. The selected areas mainly heaps and tailings ponds from uranium processing facilities represent different nuclide composition and activity levels. Specific activities of radionuclides of the U-Ra series of up to 2200 Bq/kg have been measured.


PP61

ENVIRONMENTAL DOSE MEASUREMENT WITH MICROPROCESSOR BASED PORTABLE TLD READER

S. Deme, I. Apathy, I. Feher

KFKI Atomic Energy Research Institute, H-1525, Budapest, Hungary

A new, microprocessor based thermoluminescent dosemeter (TLD) reader Pille'95 has been developed for environmental and space dosimetry. The new reader uses the same type of bulb dosemeter (TLB-2 based on CaSO4:Dy) as the earlier version of the Pille reader developed in period 1978-84.

Due to application of new electronic circuits the reader read out precision equal to 0.1 uGy, the background stability is about +-1 uGy. Each bulb is combined with a memory chip containing the individual identification number of the dosemeter. This number is automatically registered during read out process as well as the time of measurement and the temperature inside the reader. The microprocessor calculates the corrected dose and writes all date on a memory card together with the 100 channel glow curve up to 4000 measurements. The rechargeable battery operated reader weights about 2 kg.

Using the mentioned TLD system the usual environmental gamma-radiation doses can be measured with time period 2-3 days without any transport dose. As the measuring range of the system covers more that six orders of magnitude both the normal and accidental environmental doses can be measured. The portable reader significantly accelerates the availability of accidental doses.

The space version of the reader shall be used by ESA astronaut on the board of the Mir space station in second half of 1995.



PP62

ONION ROOT TIP CELL SYSTEM FOR BIODOSIMETRY?

J. Paradiz, B. Druskovic and J. Skrk *

National Institute of Biology Ljubljana, Karlovska 19, POB 141, 61000 Ljubljana, Slovenia
* Institute of Oncology, Department of Radiobiology, Zaloska 2, 61000 Ljubljana, Slovenia

Possible applicability of cytogenetic analyses of irradiated plant cells for biological dosimetry of environmental ionizing radiations was studied. The dose-effect relationships for chromosomal damages in onion meristematic cells were established after plants were irradiated and then grown in laboratory and field conditions.

Irradiations were performed on onion ( Allium cepa L.) with 60 Co gamma rays in two series of experimental plants. In the first one, 2-3 cm long roots in tap water were irradiated with single doses of 1, 3, 5 and 8 Gy at the dose rate of 1.6 Gy/min and samples for cytogenetic analysis were taken 6, 12, 24, 30, 48, 54, 72 and 78 hours after each irradiation and the control. In the second series dormant onion bulbs were irradiated with 10, 20 and 30 Gy at the dose rate of 1.8 Gy/min and samples for cytogenetic analyses were taken 6, 8, 11, 15 and 20 days after irradiated and control bulbs were planted and grown in field conditions. Squash-slides of onion root tips were prepared for cytogenetic analyses by standard methods, and the mitotic indices (MI), frequency of chromosomally aberrant cells (AC) as well as frequency of interphase cells having micronuclei (MN) were determined for each sampling time, radiation dose and the control.

The results of cytogenetic analyses in onion cells of both experimental series reveal the dose dependent relationships of MI, AC and MN but, they are statistically not significant enough to be used as biological dosimeter of absorbed radiation dose in plants from natural environments.



PP63

A WHOLEBODY COUNTER WITH SEMICONDUCTOR DETECTORS FOR RADIATION PROTECTION MEASUREMENTS

E. Lovranich, F. Steger, L. Riedlmayer

Austrian Research Center Seibersdorf, Department Radiation Protection, Austria

At the Austrian Research Centre Seibersdorf a Whole-Body-Counter with semiconductor detectors was designed and installed. The measurement geometry is the 'Scan-Geometry'. Two high-purity germanium detectors (each 30% rel. eff.) are scanning across the person, one below and the other above the person. Both detectors are shielded with a lead-shield. The wall-thickness is between 2 and 4 cm. It is also possible to use additional lead-collimators in different shapes. Physical characteristics as longitudinal, transversal and vertical variations of efficiencies were measured. Calibration measurements were done with the BGA-Phantom in different sizes and lower limits of detection were calculated. This Whole-Body-Counter is very convenient for radiation protection measurements, although the shielded room where it is situated has not extremely good low-level conditions.


PP64

DAILY AND SEASONAL VARIATIONS OF OUTDOOR ALPHA-ACTIVITY CONCENTRATION IN SALZBURG CITY/AUSTRIA

H. Lettner, A.K. Hubmer, R. Rolle, R. Winkler, F. Steinhäusler

Institute for Physics and Biophysics, University of Salzburg, Austria

Long-term continuous measurement of the atmospheric outdoor alpha-activity concentration have been performed by using a newly developed aerosol-monitor, roof-mounted 15 m above ground. The alpha-activity concentration was identified to be predominantly attributed to radon progeny. The total alpha-activity covers a range of two orders of magnitude.

Three different components of variations could be identified with regard to temporal variations: Short-term diurnal component (daily variation), mid-term component (days to weeks) and long-term component (seasonal variation). Large diurnal variations could be observed reaching up to one order of magnitude, depending on the prevailing meteorological conditions.

Variations in that time range of days to weeks are caused by to the local weather situation. Abrupt changes in the time-dependent activity concentrations reflect fast changes in the weather situation, which are characteristic for this geographical position at the northern slope of the Alps. The third component with a period of months is due to long-term seasonal variations. The diurnal component is most the pronounced, exceeding both the mid-term component due to the prevailing weather conditions and the seasonal component. The results of continuous measurements of the outdoor alpha-activity concentration over a time span of 1,5 years are presented in the paper.



PP65

PREPARATION AND INVESTICATION OF THERMOLUMINESCENCE PROPERTIES OF CaSo4:Dy,Cu

I. Kasa, J. Solymosi, A. Molnar

Technical University Budapest, Department of Physical Chemistry, H-1521, Budapest, Hungary

Calcium sulphate doped with dysprosium or thulium (CaSO4:Dy, CaSO4:Tm) has excellent dosimetric properties.

Nowadays they are among the most sensitive thermoluminescent dosimeter (TLD) materials, thus application to measuring of small dose are wide ranging. The dosimetric characteristics of CaSO4:Dy is in the dose range of 10-6-1 Gy linear, and above 1 Gy it is supralinear.

The glow curve of CaSO4:Dy has peak(s) in three temperature range: at 80- 120 C low temperature peak(s) (LTP); at 220-250 C dosimetric peak (DP); and about 350 C high temperature peak(s) (HTP). Generally the LTP in responsable for fadding, while HTP accounts for supralinearity.

Reducement of LTP can be achieved by special purification of the starting materials [1], while that of HTP is carried out by application of copper coactivator [2].

The effect of copper on the HTP of the glow curve was investigated in the concentration range of 0-0,3 mol % copper, at different Dy concentrations.

The CaSO4:Dy,Cu has been prepared - according to our method [3] - by crystallization from hot sulfuric acid containing a small amount of hydrogen peroxide.

According to the data of measurements, the HTP (the deep traps) decreased significantly and the upper limit of the linearity is increased more than one order of magnitude. Thus the application of CaSO4:Dy,Cu may be extended to the field of the accident dosimetry as well.

The results of our investigations will be discussed in detail in the presentation.

References:

  1. Kasa, I.: Rad. Prot. Dosim. 33. (1-4) 299-302 (1990)
  2. Srivastava, J.K.: Bhatt, B.C; Supe, S. J.: Rad. Prot. Dosim. 40 (4) 271-274 (1992)
  3. Kasa I.: Hung. Pat.: 197967 (Cl. G01T/11) 1990.



PP66

ELECTROCHEMICAL ETCHING OF CR-39 DETECTORS AT ROOM TEMPERATURE

G. Dajko

Institute of Nuclear Research of the Hungarian Academy of Science, H-4001 Debrecen, Pf. 51., Hungary

Different etching solutions which are suitable for an effective chemical etching at room temperature were tested.

It was found that the so called PEW solutions seemed suitable for the electrochemical etching at room temperature without any chemical preetching of detectors.

The background obtained with electrochemical etching was determined at different electrical parameters.

The sensitivity of CR-39 detectors was investigated for AmBe neutrons at different etching conditions.



PP67

IMPROVEMENT OF PERSONAL DOSIMETRY - POCKET DOSEMETER

Z. Radalj, Z. Cerovac *, I. Prlic, H. Cerovac

Institute for Medical Research and Occupational Health Zagreb 2 Ksaverska street, POB 291, Zagreb, Croatia
* ALARA INSTRUMENTS, d.o.o.

Key words: radiation protection, film dosimetry, TLD, pocket dosemeter

Film and TLD dosimetry both have a certain delay in dose reporting, since the reports on occupational doses are usually available to the users within 40 days after the actual exposure. This is particularly important when the dose is received within the short-time interval or when the radiation source has some technical failures. For that reason, the additional monitoring is recommendable. An electronic pocket dosemeter is a device which serves as an on-line exposure monitor in daily routine, making dose report promptly available to the user. The importance of this opportunity raises when significant exposure is to be expected due to the nature of work or exceptional circumstances. Such dosemeters are already available on the market , but we have developed one covering 8 main parameters such as exposure time, dose rate, dose, total dose, dose limit etc. Pocket dosemeter is to be considered the addition to the regular state dosimetry, able to complete the information on radiation exposure. In cases of any irregularities, the information is promptly reported to the health officer in charge, so that the cause can be eliminated as soon as possible. Therefore, personal film and TLD dosimetry carried out in our Laboratory has been recently improved by pocket dosemeter usage.



PP68

REMOVAL OF Ra 226 FROM WASTE WATERS ORIGINATING IN MINING AND PROCESSING OF URANIUM ORES,USING NATURAL ZEOLITES

I. C. Dutu, G. N. Sandor, T. Peic, G. Dinca

Research and Design Institute for Rare and Radioactive Metals- Research Laboratory for Radiation Protection, Working Conditions and Ecology- Petru Groza Town, Romania

The research has been done on laboratory level by using native natural zeolites in sorbtion columns. The zeolite were of clinoptilolyte type, and waste waters used have been: mine drainage waters, waste waters from radiometric sorting of ore, and tailings pond waters from a uranium processing plant.

The waste waters having contents of more than 3.7 Bq 226 Ra/liter, have been passed through simple and double columns at different flow rates and geometres of columns (height/diameter).

On the basis of the experimental results,the parameters of the procedure have been established, which enable us to obtain a radium removal efficiency of more than 95% at the passage of above 2000 BEV waste waters.

Some elution tests of radium have been effectuated, too, which have proved that natural zeolite can be used, if it is useful, in several sorbtion cycle, the efficiency of removal remaining at high values.

The analytical control of processes has been achieved by radium 226 determination (indirectly by measurement of its daughter-radon 222).



PP69

FAST NEUTRON SPECTROMETRY WITH THE STYLBEN CRYSTAL SCINTILLATOR AND PULSE SHAPE DISCRIMINATION

L.Daraban *, T. Fiat *, M.D.Croitoru *, Marta Bayer **

* Babes Bolyai University, Faculty of Physics, Cluj-Napoca, Romania
**Medical Center and Health Services and Management Cluj, Romania

We registered the neutrons spectrum emitted by a Am-241 - Be-9 source having the flux value of about 106 n/s, using a spectrometer with a 30*20 mm stilben crystal scintillator and a pulse shape discriminator device, by the charge comparison method.

This device, we build, is able to saturate the pulses generated by the gamma photons depending on their energy. So by cutting off the 4.43 MeV gamma photons the utilisation of a Cob-60 source is enough. The value of the discrimination efficiency was 5*10-4 (gamma = impulse number which get into the neutronic spectrum / number of all incident gamma photons) for a discrimination threshold get at En *= 1 MeV. The standardisation of the recoil protons spectrum was made by using the Compton electrons, generated by sources with known energies (actually we standardised with Emax = from Compton edge). This energies are turned by the luminosity function into equivalent proton energy which produce the same number of photons in the scintillator. This formula was checked with D - D and D - T neutrons.

We calculated also the efficiency of the scintillator depending on the neutrons energy and we introduced a correction factor that stands for he secondary effects which affect the recoil proton spectrum. The neutronic spectrum was extracted from the recoil protons spectrum by using a unfolding programme. The energetic groups that we established for the Am - 241 - Be - 9 source spectrum are in agreement with the reference material.



PP70

SARAD EQF 3020 A NEW MICROSYSTEM BASED MONITORING SYSTEM FOR THE CONTINUOUSE MEASUREMENT OF RADON AND THE ATTACHED AND UNATTACHED FRACTION OF THE RADON PROGENY

T. Streil, G. Holfeld, V. Oeser, Ch. Feddersen, K. Schönefeld and R. Klinke *

SARAD GmbH , Cunnersdorfer Str. 12, D-01705 Freital, Germany
*Fraunhofer-Institute of Microelectronic Circuits and Systems, Finkenstr. 61, D-47057 Duisburg, Germany

The knowledge of equilibrium factor F between the radon gas and its short-lived progeny and the change of the unattached / attached ratio is important for the risk assessment. The continuous measurement of this parameters is very difficult.

Therefore we developed a monitorsystem using separated measurement heads for the single components of the radon progeny which are in connection with an aerosol ( attached fraction ) and which are not ( unattached fraction ) by means of a filter combination consisting of screen ( mesh grid ) and glass fiber filter.

The air to be measured passes the screen and the aerosol filter in an open geometry. The filtered air goes to a measuring chamber where decay products from the radon present in the chamber volume are deposited by an electrostatic field onto the third sensor. The air is pumped every 2h for 6min. After the pump interval by automatically swivelling of the screen and one detector head start the decay detection of the on the filters collected radon progeny. The A/D converters contained in the microsystems [ Streil, et al. 1994 ] allow for a discrimination of radon, thoron and radon and thoron daughters. The monitor SARAD EQF 3020 is optional also available with three conventional 2 cm2 PIN-diodes for the alpha detection. The decay of the individual components is followed for 2h after pumping for the three sensors to calculate radon and progeny concentrations.

With this protocol we get a detection limit of about 1 Bq/m3. At 100 Bq/m3 the statistical error is below 10% ( 1s ). Dead time losses of the sensor are below 10 % for up to 106 alpha particles per second and cm2. Therefore concentrations of up to 10 MBq/m3 can be measured.

The efficiency of the radon-and progeny monitoring systems was proved in various applications like the quality control of mitigation actions .

Dresden and Freital are placed in a high radon risk area with radon concentration in buildings up to 100 000 Bq/m3. In more than 50 new and old buildings radon mitigation action are tested.

Reference:

Streil, T., R. Klinke, A. Erlebach, P. Hübler, W. Kluge, H. Kück and G. Zimmer; Sensors and Actuators A, 41-42 (1994) 85-87.



PP71

LOW-LEVEL GAMMASPECTROMETRY WITH GERMANIUM-DETECTORS: EXPERIENCE WITH A NEW CALIBRATION METHOD

P. Jachs 1, F. J. Maringer 1, M. Tschurlovits 2

1 BFPZ Arsenal, Geotechnisches Institut, Vienna, Austria
2 Atominstitute of Austrian Universities, Vienna, Austria

A new method to obtain the efficiency of a Ge-coaxial-detector in dependence of the gamma-ray energy and of the relative source-to-detector position is presented. Because of the geometry (detector and sample are of cylindrical shape) ring-shaped sources of various radii were used. For that purpose standard solutions in the energy region of 80 to 2000 keV were prepared. The spectra of these sources were measured at different positions by using detector-insets with adjustable height.

The peak- and the total-efficiency in dependence of the energy and the source-to-detector distance was obtained by numerous measurements. In order to get a mathematical expression computer aided parameter fitting was carried out.

A function of 27 parameters was found to describe the depencies of the peak-efficiency. An analogous function (25 parameters) describes the total-efficiency-dependencies. Both approaches agree reasonably well with the measured data.

The formula for the peak-efficiency epsilon is:

epsilon=a1*E**a2 * (1-exp(a3*E**a4))

where:
E - gamma-ray energy,
ai = ai (E, r, h, tan theta, s) - parameter functions
s = k0 + k1*E + k2*E2 - distance virtual point detector" - end cap
d - distance virtual point detector" - source
theta - angle between detector axis and d

These functions represent the measured efficiency data with an accuracy of only 3 % in the energy range 100-2000 keV.

This new method offers the advantage that the functions for efficiency-calibration can be generalized to any other coaxial-detector of similar measuring geometry; for fitting the parameters only a few measurements with calibration sources will be necessary.



PP72

SUM-PEAK AND 4 (PC)-GAMMA COINCIDENCES METHODS FOR RADIOACTIVITY METROLOGY AT INP OF TIRANA

Xh. Myteberi 1, A. Hoxha 2 and A. Simeqi 2

1 Institute of Nuclear Physics, Tirana, Albania
2 University of Shkodra, Albania

In the frame of a QA/QC national program, some methods of absolute measurement of radioactivity are carried-out. Starting more than 15 years ago, over 15 radioisotopes are standardized by 4 , LSC, 4 (PC)- and sum-peak coincidences methods. The most important methods are presented. One-dimensional extrapolation of efficiency for I-131 and Au-198, two-dimensional extrapolation of efficiency for Cs-134 and tracing by Cs-134 for Cs-137 methods of standardization are briefly described. The estimated overall uncertainty for the above radionuclides was better than 0.3% at 99.7 confidence level. The deviations of our results from those of solutions certified by DAMRI-Saclay have been less than 0.2%.

Thin pure Au and Mn-Cu alloy detectors are used for the absolute measurement of thermal neutron fluency at different points of activation geometry of an Am-Be source by 4 - method. The comparable respective values are given.

Due to the wide use in nuclear medicine and veterinary and the great interest of I-125 accurate measurements, the sum-peak method is recently applied. The same solutions are standardized both by our lab. and by Italian primary institute (INMRI/ENEA). Our values of their activity concentration deviated less than -0.5% from those found by Italian institute. The procedures and the corrections performed by INP are reported. Taking into account the total deviation range of 3.6% for 18 participants of I-125 intercomparison, organized by BIPM (1988) and the Italian result there (+1.2% from mean value), our bilateral comparison indirectly confirmed the correctness of our procedures and methods.

References:

  1. Xh.Myteberi Papers of INP, Acad. of Sciences,Tirana Nr1(1983),
  2. Xh.Myteberi Proceed. of 1st Balkan Phys. Union,Greece (1991),
  3. Xh.Myteberi Papers of INP,Ac.of.Sc,Tirana Nr6(1990), Nr7(1995),
  4. P.DeFelice,Xh.Myteberi Journ.Of Radioanal and Nucl.Chemistry (accepted to be published) (1995),
  5. G. Ratel BIPM Report 90/3 (1990).



PP73

SATURATION EFFECT ON ELECTROCHEMICALLY ETCHED POLYCARBONATE DETECTORS

J. Buysse, A. Poffijn, G. Meesen

I.N.W. Nuclear Physics Lab, Proeftuinstraat 86, B-9000 Gent, Belgium

It is a well known fact that radon is the most important factor in the natural radiation background. For large scale radon measurements, different types of integrating devices, mainly based on nuclear track detectors such as polycarbonate, cellulose nitrate or CR-39 can be used. For high exposures the problem of track saturation occurs. This is especially true for electrochemically etched detectors which have large track diameters.

The saturation effect of electrochemically etched polycarbonate detectors (Makrofol) has been investigated in laboratory and field conditions. Track densities of up to 4000 tracks/cm2 have been used. The tracks were counted manually on prints made with a microfiche reader. The results of these tests show a non-linear response between radonexposure and trackdensity. By correcting for this non-linearity, we showed that electrochemically etched Makrofol detectors can be used for trackdensities up to 4000 tracks/cm2.

To investigate the error on a radon measurement induced by the uncertainties on exposure time, variations in etching conditions and manual track counting, a theoretical analysis has been conducted. This analysis shows that the minimal error (1 sigma) we can expect for a radon measurement is in the order of 20 % for track densities above 400 tracks/cm2. Under 100 tracks/cm2, the uncertainty raises steeply.



PP74

CALCULATION OF THE ELECTRIC FIELD INSIDE ELECTRET IONISATION CHAMBERS - INFLUENCE ON THE RESPONSE FUNCTION

H. Stadtmann 1, L. Breitenhuber 2, P. Kindl 2

1 Austrian Research Centre Seibersdorf, Austria
2 Technical University Graz, Austria

The use of electret ionisation chambers for the measurement of gamma dose and radon exposure was increasing rapidly in the last years. In contrast to conventional ion chambers, the electric field in these detectors is not constant during the exposure time. Both field-strength and direction are changing due to inhomogeneous discharge of the electret surface charges.

Data of numerical field calculations inside cylindrical electret ionisation chambers are given. The change of the field-strength distribution with respect to electret discharge is described. The influence on the response function is discussed and experimentally verified.

The results lead to a good overview of the dynamics of the electret discharge inside ion chambers. Possibilities for optimisation of these detectors are derived.



PP75

THE LUNG COUNTER FOR "IN-VIVO" ASSESSMENT OF LOW ENERGY PHOTON EMITTERS IN LUNGS

C. Dumitru, M.A. Puscalau

Institute of Atomic Physics, Institute for Physics and Nuclear Engineering (Lab 7) Bucharest-Magurele, P.O.BOX MG-6, Romania

A lung counter installation was constructed and calibrated for the determination of small amounts of X or gamma ray photon emitters, in the energy range from 10 keV to 200 keV, which could contaminate, through inhalation, the human lungs.

The counting system consist of one phoswich detector, suitable to detect low level, low energy radiation in the presence of high background.

The scintillation sandwich is composed by a NaI(Tl) crystal, diameter 127 mm and thickness 5mm, optically coupled to a CsI(Tl) crystal, diameter 127 mm and thickness 50 mm, installed inside a steel monitoring shield.

An additional "graded Z" lining consisting of 5 mm lead and I mm copper has been added.

The phoswich detector is connected to a pulse shape discrimination electronic chain for energy selection and background reduction.

The whole system was calibrated using a male thorax phantom whose lungs were filled with standard natural uranium pellets, simulating an even distribution. The activities of the lungs were 203.350 Bq for the right and 141.624 Bq for the left. The obtained efficiency factors for the right and left lungs were 5.14310-2 imp/Bqs and, respectively, 3.49310-2 imp/Bqs.

This paper will discuss the results of background reduction and the calibration of the lung counter.



PP76

A NEW DETECTOR SYSTEM FOR DIRECT ASSESSMENT OF DOSE EQUIVALENT RATE DUE TO INCORPORATION OF GAMMA-EMITTING RADIONUCLIDES

H. Doerfel

Karlsruhe Research Center - Technology and the Environment, Karlsruhe, Germany

The conventional procedures for in vivo monitoring of gamma-emitting radionuclides involve the determination of body or organ burdens using whole body counting techniques and the subsequent estimation of intake and committed dose equivalent. For these procedures extensive information is required, such as time and pathway of intake, physical and chemical form of incorporated materials, metabolism etc. By means of routine monitoring these information become hardly available, thus resulting in significant uncertainties for the estimation of intake and committed dose equivalent.

In order to meet these difficulties, at Karlsruhe Research Center a new method for direct internal dosimetry has recently been developed. The method is based on the measurement of the integral photon flux emitted from the body using a special detector system, which has been optimized in such a way that the system sensitivity matches the respective dose factors for a maximum number of radionuclides and deposition sites in the body.

The detector system consists of four plastic scintillation detectors, which are positioned at the thyroid, at the lungs, under the gastro-intestinal tract and over the thighs of the seated person. The detector system is very easy to handle. The measurement can be performed by anybody without special training and the results in terms of dose equivalent rate are available after a very short measuring time (20 s). When performing one routine measurement per week, the lower detection limit is less than 0.1 mSv/a and the mean detection uncertainty is about 20 % for known radionuclide mixtures, and about 60 % for unknown radionuclide mixtures.



PP77

A METHOD FOR CALCULATING THE SPATIAL DISTRIBUTION OF RADIOACTIVITY MEASURED BY A WHOLE BODY COUNTER

G. Greifeneder 1, H. Aiginger 1, F. Steger 2, E. Unfried 1, L. Riedlmayer 2, H. Havlik 3, H. Bergmann 3

1 Atominstitute of the Austrian Universities, A-1020 Vienna, Austria
2 Austrian Research Center Seibersdorf, A-2444 Seibersdorf, Austria
3 Department of Biomedical Engineering and Physiks, University of Vienna, A-1090 Vienna, Austria

The detector system of the high sensitive whole body counter consists of four 8"x4"-NaJ(Tl) crystals with multi-slit focused collimators inside a massive shielding chamber. Two of these linear scanning detectors are placed above and two below the bed. They can be arranged independently in three dimensions. A pressedwood phantom was constructed to simulate different point source positions in the human body.

To achieve spatial resolution a special detector configuration was chosen. Using different point source positions linear profile scans were measured systematically for various radionuclides (133Ba, 131J, 22Na, 137Cs, 60Co) over a wide energy range. Based on these data a model was developed. This model allows to determine an unknown position of a point source in the pressedwood phantom and can be easily extend to medical applications.



PP78

ACREM: THE AIR CREW RADIATION EXPOSURE MEASURING SYSTEM

P. Beck, K. Duftschmid, St. Kerschbaumer, Ch. Schmitzer, Ch. Strachotinsky

Austrian Research Centre Seibersdorf, Austria

Because of new recommendations of the International Commission on Radiation Protection ICRP60 the natural exposure in civil aviation should be take into account. An update of the quality factors for neutron radiation increases the quota for the neutron component of the equivalent dose of about 60% compared to values of ICRP60. Numerous exposure measurements at civil airlines in Sweden, USA, Russia and Germany show a radiation exposure in the range of 5 - 10 mSv/year. This is clearly more than the average annual dose of occupational radiation workers (in Austria about 1.5 mSv/year).

An economical and simple method to record the radiation exposure is realised by a combination of measurements with a reliable gamma dose rate instrument (SSM-1, Radiation Measurement System of Seibersdorf) and using a software algorithm. Operating a GPS (global position system) in addition the energy spectrum of the cosmic radiation, depending of the geographical position and altitude and from this the total radiation exposure of the air crew is achieved. Uncertainties because of statistical events of solar flares or the changing of altitude and route of the airline can be excluded compared to calculation models only of radiation exposure determination.



PP79

AUTOMATIC SYSTEM FOR CONTINUOUS MONITORING OF GAMMA ACTIVITIES IN ATMOSFERIC PARTICULATE

M. Montalto, R. Giacomelli, M. Nocente, S. Bortoluzzi, P. Spezzano

ENEA, Dipartimento Ambiente, AMB-ICR-TER CR Saluggia, Italy

This paper describes the design criteria, which were used for the realization of an automatic system for the real time monitoring of the artificial radioactivity in the air.

The air monitoring system includes:
- air sampler;
- spectra acquisition system;
- computer and various peripheral units.

The air sampler is formed by a filter holder and a suction unit.

The filter holder is directly mounted on the high-purity germanium detector, and was designed so as to optimize both the flow rates of filtered air and the detection geometry of the radiations emitted by the radionuclides eventually present.

Special attention was paid to minimize particulate losses along device ducts. Particulate losses showed to be lower than 10%.

The designed automatic monitoring system allows to carry out the monitoring of air radioactivity complying with the same operating parameters, which are used in the traditional manual procedure. The minimum detectable activities and the particulate-collection showed, in every respect, to be equivalent to the traditional system.

In addition, it allows to reduce, even to few minutes, the time intervals between different measurements and, therefore, a continuous alarm system is available.



PP80

MANUAL TLD SYSTEM FOR MULTIPLE DOSIMETER FORMS AND APPLICATIONS

R.A.Tawil 1, K.J.Velbeck 1, J.Fellinger 2, R.Plompen 2, M.Majewski 2

1 Harshaw/Bicron Radiation Measurement Products, 6801 Cochran Road, Solon, OH 44139, USA
2 Bicron Technologies Vertriebs-GmbH, Viktoriastrae 5, 42929 Wermelskirchen, Germany

This paper describes and reports the performance of a new manual TLD system that reads all forms of TL materials for a wide variety of applications. The system is composed of a two-PMT Model 4500 TLD reader, advanced dosimeters, automatic QC Glow Curve Analysis, and Neural Network dose algorithm.

The TLD reader incorporates independent dual hot gas and single planchet heating methods integrated into one drawer. This supports the reader's use in such diverse applications as external whole body and extremity personnel dosimetry, medical physics, environmental monitoring, spice and food irradiations, archeological and high dose dosimetry. The various dosimeters include card-mounted chips in symmetric and non-symmetric holders, high sensitivity LiF:Mg,Cu,P material, rods, microcubes, and powder.

Application software to perform data acquisition and storage, Calibration, Quality Assurance and Control, automatic glow curve analysis with identification of irregularities and neural network-based algorithms is layered on the system to provide building blocks for increased capability.

Test data presented in this paper include sensitivity, linearity, minimum delectability, repeatability, residual effects, ambient light sensitivity, glow curve analysis and algorithm performance.



SESSION V:
NON-IONIZING RADIATION


OP43

THE NEW EUROPEAN TEHNICAL STANDARDS ON THE HUMAN EXPOSURE TO ELECTROMAGNETIC FIELDS

A.A. Russo

Italian National Research Council, Dept. of Prevention and Work Safety, Rome, Italy

In the 1995 the European Prestandard CENELEC ENV. 50166 was approved and promulgated. This technical standard is oriented to establish the methodology for the protection of the workers and the general public against the risks, due to the exposure to electromagnetic fields in the range of frequency from O Hz up to 300 GHz. The prestandard is divided in two different parts; the first one regards the low frequency range from 0 Hz up to 10 kHz and the second one the high frequency range from 10 kHz up to 300 GHz. This is a prospective standard for provisional application so gain experience in its use. In this prestandard the following main arguments are considered: the exposure limits, both for the workers and the general public, the methods of measurements, the rationale for the setting the limits. The scope of the standard is the prevention of the adverse short-time effects on the human beings from the exposure to electromagnetic fields, with particular regard to the methodology for their evaluation from protection point of view. In the present paper the author want to show the principles of the prestandard and to make a possible evaluation of the potential impact, due to its application, on the research, industrial and medical fields both from technical and economical point of view.


OP44

HIGH VOLTAGE POWER LINES IN ITALY: QUANTITATION OF EXPOSURE AND HEALTH RISK EVALUATION

C. Petrini, A. Polichetti, P. Vecchia

Physics Laboratory, National Institute of Health, Rome, Italy

New regulations have recently been proposed in Italy, both at national and regional level, aimed at preventing possible long-term health effects of magnetic fields from power lines. Based on some indications from the epidemiological literature, the proposed standards require the exposure limits to be reduced to values that are three orders of magnitude lower than recommended by IRPA/INIRC guidelines. Such drastic action obviously involves high economic and social costs, and a careful cost/benefit analysis is therefore required prior to the enforcement of new standards. As a basic input for such analysis, a quantitative estimate of health risks has been performed, based on detailed data on the distribution of population around power lines. This kind of data are generally not found in the literature and are now available in Italy as the result of an extensive survey performed by the national electrical utility, ENEL. Estimates of excess cancer are presented, which are based on risk factors given by the most recent and large epidemiological studies.


OP45

ASSESSMENT OF MAGNETIC FIELDS EXPOSURE FROM AC POWER LINES IN AN ITALIAN RESIDENTIAL AREA

S. Tofani, G. d Amore, G. Fiandino, M. Tasso

Servizio di Fisica Sanitaria, Azienda USL 9, Ivrea, Italy

Results of narrow- and broad-band measurements of the Magnetic Flux Density (MFD) inside and outside houses located close to a 380 KV double circuit power line are reported together with the correspondent calculated values. The survey lasted 3 months with week-long continuous MFD measurements. The monitoring of the current flowing in the line was also provided. The agreement between calculated and measured MFD values is within 10%. The MFD assessment accuracy was within 8% either by taking the metre maximum reading (or by measuring the three orthogonal components). The maximum harmonic component has been always below 1.3% the fundamental. The front door MFD measurement can give a good estimate of the exposure inside the house depending on the house position in respect to the line. The time and seasonal variation of the exposure was estimated about 25%.


PP81

THE ITALIAN NATIONAL ARCHIVE OF RADIO AND TV BROADCASTERS: PRELIMINARY EVALUATIONS OF HEALTH AND ENVIRONMENTAL IMPACT

V. Lepori 1, A. Polichelli 2, P. Vecchia 2

1 PMIP Dept. of Physics and Environment Protection - USSL 5, Como, Italy
2 Physics Laboratory, National Institute of Health, Rome, Italy

Experimental surveys performed by a number of health authorities in Italy have shown that in several cases electromagnetic fields radiated by antennas for radio and TV broadcasting exceed exposure limits recommended by international organizations such as IRPA/INIRC, or set by regional standards in some Italian regions. As a basic tool for a nationwide control of the health and environment impact of such plants, a national archive of broadcaster in Italy has been designed and developed.

From the main archive, installed on PC, regional subsets may be extracted, which are managed by the same application program, developed both for MS DOS and Macintosh. The data refer to 27,332 radio and 28,769 TV broadcasters, for a total of 56,101 plants, a number probably higher than in any other country. Preliminary analyses of data provide important information on the distribution, both geographical and for class of power, of emitters. A detailed comparison of distribution of antennas and population has been made, limited for the moment to the region Lombardy. Similar analyses are being performed in other Regions, which are likely to be involved in the same kind of problems.



PP82

EVALUATION OF RECOMMENDATIONS ON LIMITS OF EXPOSURE TO ULTRAVIOLET ON THE BASIS OF DATA FROM THE AUSTRIAN POPULATION

G. Keck, G. Schauberger, A. Cabaj

Institut für Medizinische Physik, Veterinärmedizinische Universität Wien, Austria

For the application of solaria at present the following international recommendations on limits of exposure exist, which differ strongly:

1. IRPA/INIRC (1991): 30 MED/a;
2. IEC 335-2-27 (1978, 1989): 25 kJ/m2/a for each region of the body, that is 100 MED/a.

On the basis of our data from the Austrian population (1) we can give an evaluation of the recommendations for a whole population.

For the Austrian population older than 16 years we found for 1990 a mean UV-exposure of 53 MED (22 MED for work outdoors, 29 MED leisure time and holidays, 1.5 MED solaria). A demographic analysis shows, that the mean UV-exposure of more than of the Austrians is below 38 MED/a. Highly exposed groups are outdoor workers (>4 h/d) with 125 MED/a, persons exercising summersports outdoors and spending their holidays at the Mediterrian (84 MED/a) and the user of solaria (79 MED/a).

Only 9.8 % of the Austrian population use solaria. A frequency distribution of skin dose shows, that 80 % of them do not reach 30 MED/a, less than 1 % exceed 100 MED/a. The recommendation of the IEC therefore is much too high, it seduces rather to use solaria than to restrict their application. We recommend to adapt the international standard IEC 335-2-27 to the IRPA/INIRC recommendations, so that irradiation schedules on the basis of an annual dose of 7.5 kJ/m2 and skin area (that is 30 MED/a) should be drawn up.

Reference:
(1) Keck Gertrud, Cabaj A., Schauberger G. (1992): UV-Exposition der Österreichischen Bevölkerung durch solare Strahlung in Beruf, Freizeit und Urlaub sowie durch die Nutzung von Solarien, Hrsg. vom Gesundheitsministerium für Gesundheit, Sport und Konsumentenschutz.



PP83

SECONDARY HAZARDS OF HIGH POWER LASER BEAM WELDING

K. Schulmeister, C. Schmitzer

Austrian Research Centre Seibersdorf, Austria

With laser materials processing, direct exposure to the laser beam is usually not the main hazard. The high power laser beam is enclosed up to the surface of the workpiece and is usually directed towards the ground. Errant beams can be caused by uncontrolled reflections off the workpiece surface, however this happens rarely and protection is generally afforded by shields around the workstation.

Secondary hazards such as UV-radiation, ozone and fume produced by the laser-workpiece interaction are more serious due to the every-day, long term exposure of the worker.

In this paper, an overview will be given of the secondary hazards associated with C02 laser welding. The UV-radiation emitted by the high temperature plasma above the welding-keyhole and the ozone and NOx production due to UV-induced photodissociation of oxygen and high temperature gas-phase reactions will be discussed. Spectral measurements of the plasma emission showed that the allowed dose for UV-radiation and blue light exposure per work day can be exceeded in as short as a few seconds. Similarly, measurements and models of the ozone and NOx concentration showed that the maximum workplace concentrations might be reached quickly if no appropriate exhaust and filter system is installed.



SESSION VI:
RADIATION PROTECTION AND THE SOCIETY


OP46

IAEA POLICY AND PROGRAMME FOR EDUCATION AND TRAINING IN RADIATION PROTECTION

K. Skornik

International Atomic Energy Agency, Division of Nuclear Safety

The paper presents the main policy directions and programme for education and training in radiation protection and nuclear safety, as part of the IAEA s long standing commitment to promotion of occupational health and safety through manpower development in Member States. Radiation protection and nuclear safety are primarily a national responsibility. Many developing Member States still find it difficult, however, to set up and/or implement manpower development programmes, due to budgetary constraints, shortage of qualified teachers and other deficiencies in infrastructure. There is a persistent need for assistance in many areas of radiation protection and nuclear safety given the fact that nuclear methods which lead to electricity generation and improvements in food production, health care, industry and hydrology, are increasing in number and are often competitive with other methods. The aim of the Agency s assistance is to strengthen the relevant part of national infrastructures. Manpower training receives much attention in this strategy with the objective of achieving national self-sufficiency.

The guidelines for planning Agency activities in this respect are based on systematic analyses of Member State needs, and comprise concentration and standardization of efforts to assure both the highest possible standard and cost-effectiveness of the programme delivered. The programme reflects the differences amongst Member States in their radiation safety infrastructures and commitments to nuclear technologies.

For education and training activities, it is structured at three geographical levels (interregional, regional or national). The modalities include:

- Post-graduate educational courses in radiation protection (in Arabic, English, French, Russian and Spanish)
- Post-graduate educational courses in nuclear safety (in Russian and Spanish)
- Specialized training courses/workshops on selected aspects of radiation protection/nuclear safety (interregional/regional/national).

Other mechanisms comprise: fellowships, scientific visits, seminars and educational/training material.



OP47

THE RADIATION PROTECTION PROGRAMME OF THE EUROPEAN UNION AND THE ROLE OF UIR (INTERNATIONAL UNION OF RADIOECOLOGY)

A.A. Cigna

Fraz. Tuffo, I-14123 Cocconato (Asti), Italy

The starting and the development of the Radiation Protection Programme within the European Community are here described. Such a programme undervent an evolution as a consequence of the results achieved and the needs arising. Some data describing such an evolution are here reported.

The main features of the 4th Framework Programme 1994-1998 concerning the Radiation Protraction are also considered.

The role played by the International Union of Radioecology (UIR). which was founded in 1978, both in the past and in the present situation is acknowledged and the results obtained by the cooperation among different groups of scientists and other institutions are emphasized.



OP48

THE NEW ITALIAN REGULATIONS IN MATTER OF RADIOPROTECTION

L. Frittelli, R. Mezzanotte

National Agency for Environmental Protection - ANPA, Roma, Italy

Recently, in March 95, a new "Legislative Decree" was adopted, for the implementation of six UE Directives, about radiation protection of the population, of workers and of the environment.

In the paper the general outline of Decree will be presented, and some particular aspects of the Italian regulation will be discussed.



OP49

MONITORING PROGRAMME ARROUND NUCLEAR POWER PLANT KRSKO

R. Martincic 1, U. Miklavzic 1, M. Kanduc 2, S. Lulic 3, J. Kovac 4

1 Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia
2 Institute of Occupational Safety, Bohoriceva 22a, Ljubljana, Slovenia
3 "Rudzer Boskovic" Institute, Center of Marine Research, Bijenicka 54, Zagreb, Croatia
4 Institute for Medical Research and Occupational Health, Ksaverska cesta 2, 41000 Zagreb, Croatia

The off-site monitoring system is briefly described and some illustrative results concerning pollution of the river Sava, drinking water, foodstuffs and external radiation are presented. Conservatively estimated dose burdens received by a member of the reference population group as a result of NPP emissions amount to values of "the committed effective dose equivalent" smaller than 10 uSv per each year of operation. This value represents less than 0.5% of the annual dose received on average from natural and artificial sources by a member of the general public in the "normal" environment. The dose estimates concerning NPP have been performed since 1982 on the basis of emission data as well as off-site environmental measurements.


OP50

RADIOLOGICAL PROTECTION PROGRAM AT KRSKO NPP

B. Breznik

Nuklearna Elektrarna Krsko, 68270 Krsko, Slovenia

Krsko NPP, a Westinghouse two-loop PWR of 632 MWe power, is in commercial operation since 1982. Reduction of radioactive releases to the environment and the reduction of doses to workers is basic goal in the plant radiological protection. The radiation protection program is established to ensure that the radiation exposures to workers and members of the public are minimized according to the As Low As Reasonably Achievable approach and controlled in accordance with international safety standards and Slovenian regulations.

The basis for the operational and technical measures is provided by the Radiation Protection Manual and ALARA Manual. The effluent control is based on the Standard Radioactive Effluent Technical Specifications, and environmental surveillance is established according to the program defined by the regulations. The dose constraints and performance indicators are used to assure the effectiveness of the radiation protection program and provide a convenient follow-up tool.

The monitoring program results of each year show that there is no measurable dose to the public due to radioactive releases. The commitment to the dose burden of any member of a critical group is assessed to be below the dose constraint. Individual and collective doses of the workers are within a range typical for the PWR's of a similar type.



OP51

ENVIRONMENTAL RADIOLOGICAL MONITORING AROUND TRIGA REACTOR

B. Pucelj

Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia

Reactor centre Podgorica, belonging to J. Stefan Institute, is located about ten kilometres from Ljubljana. The main facilities, concerning sources of radiation, are: experimental reactor TRIGA Mark II, radiochemical laboratories and the temporary storage facility for low and intermediate radioactive waste. The radiological influence of the centre on the environment is estimated by measurements according to a special monitoring programme. The backbone of the programme are two kinds of measurements: the control of emissions and immissions. The control of releases of radioactive aerosols and gases to the atmosphere is performed by continuous measurements of the releases from the stack of the reactor. Liquid releases from radiochemical laboratories to the river Sava are controlled by taking samples and measuring the isotopic concentrations prior to the release. Several measurements and controls are done to evaluate the immissions to the environs. It is estimated that the highest dose to the nearby population is lower then about one Sv for atmospheric and liquid releases.


OP52

EMERGENCY PREPAREDNESS IN SLOVENIA

R. Martincic, M. Korun, B. Pucelj, B. Usenicnik *

Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia
* Administration for Civil Protection and Disaster Relief, Ljubljana, Slovenia

Historically, accidents have occurred during the production, transport and use of the radioactive materials. Experience has shown that advance emergency planning is essential in order to mitigate the consequences of accidents.

The paper presents the general philosophy applied in Slovenia to the problem of emergency response; background information on the Slovene nuclear power plant and nuclear energy programme; experiences in the light of the recommendations provided by the international bodies; and finally legal, organizational, planning and reviewing aspects of the Civil Protection Organization applying to radiological emergencies.



OP53

EFFECTIVENESS TESTS OF RADIATION DETECTION SYSTEMS FOR VEHICLES CARRYING SCRAP METAL

M. Fabretto, S. Colonnello, V. Barbina

CRAD, Centro di Ricerca Applicata e Documentazione, Udine, Italy

Radioactive sources accidentally mixed in scrap material and then melted in the steel process caused numerous incidents in the last years, resulting in significant levels of contamination of the steel making plants and posing serious safety problems for employees and the general public. In order to prevent this risk several companies developed radiation detection systems specially designed to detect the presence of gamma-emitting radioactive sources buried in scrap carried by railcars or lorries.

These systems generally consist in two or more detector assemblies located on the two sides of the railcars or lorries approach. The detectors are connected to a computer-controlled alarm system which usually includes special diagnostic and sensitivity controls. However the overall effectiveness of the system, in terms of high sensitivity-i.e. high detection probability of low activity sources - and low false alarm rate, depend on a strict initial test procedure and subsequent correct routine checks. In this connection different acceptance protocols based on a number of sensitivity tests and false alarm rejection checks have been proposed, e.g. by the American Institute of Scrap Recycling Industries and, most recently, by the Italian Health Ministry.

CRAD, being charged of the installation and management of a radiation detection system for vehicles carrying scrap metal on behalf of a steel industry in North-East Italy, is gaining a sound experience in applying the acceptance protocols and assessing the error probability figures vs. minimum detectable activity and vehicle speed, which is presented in this work.



OP54

RADIOMETRIC CONTROLS OF CONTAMINATED SCRAP METALS IMPORTED IN ITALY, TECHNICAL AND REGULATORY FEATURES

F. Dobici, S. Piermattei, A. Susanna

National Agency for Environment Protection, ANPA, Roma, Italy

For years there have been sporadic reports of incidents from trafficking of scrap metals radioactively contaminated or containing radioactive sources. However recently there have been an increase of events indicating that this problem is so growing as to generate possible consequences, from a radiation protection standpoint, to workers and to the public.

Following several detections of contaminated scrap metals in some recycling industries and in some consignments entering the italian boundaries, the competent Authorities laid down rules to put under control the problem.

In this paper technical and regulatory features are discussed.



OP55

A CASE OF A FOUND RADIOGRAPHIC SOURCE

B. Pucelj, M. Korun, D. Kavsek, Z. M. Rosman, T. Sutej 1

Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia
1 Health Inspectorate of Republic Slovenia, Ljubljana, Slovenia

Significantly elevated dose rate was measured locally outdoors in a metal producing facility. Further measurements by in-situ gamma spectrometry revealed that it was due to radiation from 137Cs with the activity of the order of tens of GBq, most probably from an unaccounted radiographic source buried in the soil about 10 to 20 cm deep. Since the source was located at a place where it did not present any immediate health threat to the population or to the workers of the plant its removal was carefully planned to minimize the dose to the team involved. The source was successfully recovered and safely stored in the temporary storage facility for low and intermediate radioactive waste of Slovenia in Reactor centre near Ljubljana. Although the capsule was partly corroded no soil contamination was detected. The highest dose to a member of recovery team was 50 uSv.


PP84

THE RADIOMETRIC CONTROLS ON METALLIC SCRAPS

R. Delia, A. Moccaldi, G. Barone Adesi

Ministry of Health, ISPESL (National Institute of Prevention and Work Safety), Rome, Italy

The risk connected with metallic scraps is a relevant problem from the radioprotection point of view, as the presence of detected contamination and radioactivity on stocks of these materials imported from European Eastern Countries has shown.

Consequently many controls have been carried out on the imported metallic scraps at the boundaries. These radiometric surveys have shown the possibility of presence of contaminated material in the imported stocks. The measurements have been carried out both on every road and railway load, coming from extra-European Community Countries, for fifteen months. The detected values of the radioactivity outside of the scrap containers resulted greater than the radioactivity background value, with a variable frequency between 0.1% and 1% of the surveyed loads. The presence of the radioactivity in the scraps gives born so to an health radiological problems both for the workers and for the population. In fact during the recycling processes of the scraps the worker can be exposed to undue radiation levels, greater than the background level and the population can be exposed to the same levels in the utilization of the products obtained by the recycling processes. In the present paper the author shows the obtained results in the carried out survey and the Italian promulgated legislative safety measures, in reason to prevent the possible risks connected with this kind of work. These measures are charged to the utilizing person of the scraps, to the Central and regional Authorities.



PP85

CAN COMPLIANCE WITH A LIMIT BE ASSURED BY MEASUREMENTS?

M.Tschurlovits *)

Atominstitute of Austrian Universities, Vienna, Austria

Usually, figures are set by authorities to control doses from controlled sources (normal operation ) or from sources not under control ( in emergency cases ). Such figures might be called reference levels, action levels, limits etc. and are conceptually expressed in terms of effective dose. For practical reasons, some derived quantities as activity concentration in a given substance, e.g. in foodstuffs are used, obviously assuming a given model.

In any case, an apparently very precise figure is established and compliance has to be achieved by measurements whether or not the considered figure is consistent with the limit.

Two figures with different properties have to be compared: a constant number on the one hand and an estimated value with a confidence interval on the other hand

The most frequent case is to check the question whether an activity in the sample is less than or equal to a preselected limit.

It is proposed to consider a sample in compliance with the limit when the following condition is fulfilled:

A+N*sigma <= L

where:
A...activity concentration determined by measurement
n..number of standard deviations, chosen as 1
s....standard deviation of the measurements
L.. limit

The concept is discussed in more detail in the paper.

*) The concept presented here was developed and discussed in the subgroup "Low Level measurements" of the Austrian Standards Institute (NORM,) Radiation protection branch. Members of the Working Group are: H.Friedmann, E.Henrich, P.Kindl, A.Leitner, F.J.Maringer, F.Steger, M.Tschurlovits (chairman), E. Unfried, G.Winkler



OP56

THE REGULATORY SYSTEM OF MONITORING WORKERS IN GERMANY FOR INTAKES OF RADIOACTIVITY WITH SPECIAL REFERENCE TO THORIUM

A. Dalheimer 1, K. Henrichs 2

1 Institut für Strahlenhygiene, Bundesamt für Strahlenschutz, D-85764 Oberschleiheim, Germany
2 Zentrales Referat Strahlenschutz, Siemens AG, D-81730 München, Germany

In Germany, the working group "Incorporation Monitoring" of the Radiation Protection Association defined a new standard for the monitoring of workers occupationally exposed to radioactive material. During the last two years this draft has been accepted by the German government in the form of three guidelines.

The purpose of the approach was the installation of a system:

- defining clear criteria for the necessity of regular and special monitoring programs,
- giving guidelines for monitoring programs ensuring that dose assessments are reliable as necessary with the lowest possible expenses,
- standardizing as far as possible the procedures of dose assessments, and
- guaranteeing the necessary of quality standards.

The most important features of these regulations will be discussed in this contribution and their application will be exemplified for the specially difficult monitoring of thorium intakes.



OP57

RADIOLOGICAL PROTECTION IN A NON-NUCLEAR COUNTRY

C. Hone

Radiological Protection Institute of Ireland, Dublin, Ireland

Since 1997 Ireland has operated a licensing system to regulate the use of ionising radiation in medicine, industry and education/research. The system extends to all sources from irradiators containing petabecquerels of cobalt-60 to veterinary x-ray units.

Licences in respect of radioactive materials and irradiating apparatus are issued by the Radiological Protection Institute of Ireland which is the national competent authority for matters relating to radiological protection. The licences include conditions which must be upheld by the licensee. These conditions place an obligation on the licensee too, among other things, maintain and service licensed items, calibrate dose measuring equipment, investigate and report to the institute all doses in excess of prescribed action levels (which are always lower than statutory limits). They, also specify limits for radioactive waste disposal. The institute carries out inspections of licensees to ensure compliance with these conditions and other regulations pertaining to ionising radiation. This paper will discuss the experience gained in operating the licensing system. In particular it will address the following issues

  1. ensuring quality control in medical applications.
  2. radioactive waste disposal.
  3. the use of x-ray equipment by practitioners of alternative medicine (eg. chiropractors).

The paper should have particular relevance for other small countries, particularly those without nuclear power or very limited nuclear programmes, which are in the process of developing or reviewing their arrangements for the monitoring and surveillance of sources of ionising radiation.


OP58

COMBINED LOW- AND HIGH-DOSE IRRADIATION AND ITS INTERPRETATION FROM THE POINT OF VIEW OF RADIATION PROTECTION

M.Beno

Institute of Preventive and Clinical Medicine, Limbova 14, 83301 Bratislava, Slovakia

The adaptive response after low dose irradiation attracted much attention in the last decade. It was already used as an example in advertising the "hormetic" effects of low dose irradiation (Luckey,T.D : Radiation Hormesis, p.85, C.R.C. Press Inc., 1991, 306 p). The work reported aimed at gaining information about the frequency of observation of the adaptive response in a human population sample.

In our experiments we counted chromosomal aberrations and micronuclei in human lymphocytes after a combination of low-dose irradiation with tritium and high-dose irradiation with gamma rays from a 60Co source. Three types of response could be revealed by biometric testing: additive, adaptive and synergic. The testing leads us to suppose a normal distribution of the clastogenic effect in samples of lymphocytes taken from a healthy adult population, the most lymphocyte samples responding additively and the adaptive and synergic types of response being at the extreme ends of the distribution. The occurrence of these extreme types of response depends upon the magnitude of the first, low dose and their expression may be limited to a narrow dosage-interval. A high interindividual variability prevented to estimate an "optimal" low dose which would allow in future to assess one of the extreme types of response in every individual.

From the point of view of radiation protection it is important to take into account the possibility of a synergic response after combination of two (or more) doses of radiation, especially in the low-dose region. This needs further attention to pay as the contemporary limits are accepted under the premise of additive effects of repeated doses, but, the question arises if the limits include an acceptable safety margin for individuals whose tissues may react synergically.



OP59

RADIOACTIVITY IN THE SCRAP RECYCLING PROCESS: RADIATION PROTECTION ASPECTS AND EXPERIMENTAL MONITORING PROBLEMS

D. Sacco, R. Delia, G. Bindi, A. Bonanni, S.Casciardi, Loppa, F. Marena, P. Rossi, F. Ruggeri, L. Venturini

ISPESL, Via di Fontana Candida N01, Monteporzio Catone, Roma, Italy

The steel scrap recycling by iron and steel industry is increasing mouved by profits and by the purpose of protection of environmental resources. Besides the use of radioactive sources in several fields (medical, industrial and in scientific researches) on one hand, and the disposal of made radioactive materials from nuclear reactors on the other hand, makes the likelihood no more negligible that some radionuclides could be found, accidentally or fraudulently, in steel recycling scrap. Radiation protection problems for surveillance both of employees in the production cycle and of people and environment in general arose.

First of all, we characterize different kind of radioactive materials that can found in scraps, pointing out the potential hazards from exposure of workers and people and from environmental contamination, related to physical, chemical and geometrical specifications of the involved radionuclides.

The suitable monitoring systems for scrap recycling facilities are presented considering the different phases of production cycle (transport, storage, manipulation, melting ... ).

At least, experimental data, taken in some periods of the monitoring campaign made at the Italian border on imported scraps, are presented. In particular, we point out the comparison on experimental data taken with different portable detector of different technical specifications.



OP60

EVALUATING THE SHORT-TERM RADIOLOGICAL CONSEQUENCES OF RELEASES IN ACCIDENT SITUATIONS

S. Renier

EDF, Industrial Safety, Radioprotection and Environment Department, Environment Group

One of the operator's fundamental missions is to evaluate the maximum potential volume of radioactivity which may be released, estimate the environmental impact, very rapidly carry out initial measurements at the site and outside the site, taking into account the wind factors, and transmit the results of all these evaluations to the local authorities.

1. METHODS USED BY EDF'S TECHNICAL TEAMS


The radiological consequences of an accident are evaluated using a three-pronged method:

- Determine, from the very first phase of the accident, the envelope of foreseeable releases. The estimated evaluation of potential releases and doses likely to be discharged during the accident can be obtained very rapidly.
- Track the development of releases through the stack, then calculate the radiological impact of these releases according to current meteorological conditions. These results are the compared with the values forecast.
- Interpret initial results of measurements taken in the field. These measurements taken in the area around the site are compared with the forecast results. This makes it possible to confirm or modify forecast developments and / or identify any abnormal leaks from the containment which were not recovered by the ventilation systems.

EDF specialists apply this method in accordance with a guide entitled "the Health Physics Control Center work tool", which details the three components in the evaluation process.

A computer program has been developed to help the Health Physics Control Center teams in their work. The package is known as GEEE (Gestion des Effluents et de l'Environnement), or management of effluents and the environment.

2. GEEE SOFTWARE PACKAGE


The GEEE program is a value-added tool, ensuring.

- Data collection (concerning the installation, meteorological conditions and environmental measurements).
- Automatic-real-time calculation of releases at the stack.
- Precision readings of impacted zones thanks to a puff atmospheric diffusion model. This precision is important since it both enables determining exactly where radioactivity measurements must be taken in the field and also better defining priorities for implementing measures to protect the public, if deemed necessary.
- Automatic delivery of evaluation results in the form of tables or maps.
- The possibility of determining at any given moment the radioactivity levels measured in the environment at all nuclear power sites, using the nationwide GEEE system.



OP61

RECENT DEVELOPMENTS IN RADIOECOLOGY

M.Tschurlovits

Atominstitute of Austrian Universities, Vienna, Austria

The international development of the field "radioecology" in the last decade is presented. The development can be separated into two groups: measuring programs dealing with the assessment of activity concentration in environmental compartment on the one hand and modelling activities on the other hand. Model validation exercises are going on. Programs dealing with retrospective dose assessment are discussed. Experience gained in participation in the IAEA VAMP program , river subgroup are discussed.

Both assessment and modelling are going to become more developed. Examples of these activities are presented. The present developments lead to the conclusion the existing problems can be solved only by cooperation of measurement and modelling groups. This collaboration is important for not to leave the field to groups, directed by politicians seeking for short term gain, in order to give retrospective justification in a specious manner of decisions not be based on objective analysis.



OP62

ILLICIT TRAFIKING OF NUCLEAR MATERIAL IN HUNGARY, REGULATORY AND OPERATIONAL ACTIONS IN THE FIELD OF RADIOLOGICAL HEALTH

S. Pellet, L. Ballay

National Research Institute for Radiobiology and Radiohygiene, Budapest, Hungary

Illicit trafficking of various nuclear material has been arisen in Europe as well as in Hungary in the past few years as a curiosity. This unexpected phenomenon stressed the radiation protection authorities to overview the regulations and operational guidance for radiological health actions relating to found or seized nuclear and/or radioactive materials by security organizations. The main radiological health features of Hungarian incidence will be introduced also the actions were taken in National Institute for Radiobiology and Radiohygiene and in National Radiological Health Emergency Service. Also the frame of the coming new regulation relating to radiological health responsibilities in case of found or, seized nuclear materials.


OP63

CONSIDERATION OF INHOMOGENEOUS RADIATION FIELDS FOR RADIATION PROTECTION MEASURES

M.Tschurlovits

Atominstitute of Austrian Universities, Vienna, Austria

Radiation protection standards define clearly figures limiting the radiation exposure of groups, e.g occupationally exposed persons, in terms of the quantity E (effective dose), being a quantity defined by ICRP for risk estimation, is used.

Regarding external exposure, the measurement has to be done by means of operational quantities as defined by ICRU.

There is a dichotomy between the two lines of development, and some discussions on this issue was carried out /De 94, Le 93/.

Another issue is, however, not discussed at all in the present discussion: a possible spatial inhomogeneity of the radiation field. This problem is existing in many practical cases as inhomogeneous shielding, slits im walls etc.

No information is available on the size or radiation field to be considered in a radiation survey and to set in relation with the limitation quantity.

This paper is concerned with two approaches to assess compliance with limits for spatial inhomogeneous exposure conditions. One approach is based upon judgment of measuring results, the other with compliance with limits.

References:

/De 94/ J.A.Dennis, R.V.Griffith: Rad.Prot.Dos. 54 (1994)373.
/Le 93/ A.Leitner, M,Tschurlovits: Proc. Au-Hu-It Radiation Protection Symp. Obergurgl(1993), Vol III p.386



OP64

NEW ORGANIZATIONAL FRAMEWORK OF THE RADIATION PROTECTION IN THE CZECH REPUBLIC

V. Klener

Centre of Radiation Hygiene, National Institute of Public Health, Prague, Czech Republic

The field of Radiation Protection has been developing in the Czech Republic since the early nineteen- fifties as a specific branch of Occupational Medicine. Later its scope increased to cover environmental problems and Radiation Protection became an autonomous field in Public Health. The executive framework was structured on the lines of Soviet Hygiene Service. After the fundamental political changes of 1989 the Hygiene Service has undergone substantial transformation and Radiation Protection is no longer considered a typical branch of Public Health. Accordingly the then Atomic Energy Commission of the Czech Republic has redefined its role and become a State Office of Nuclear Safety. Following the current tendency of International Governmental Organizations to bring closer the protection of health and the safety of radiation sources - as expressed in the International Basic Safety Standards (1994) - both these activities have been entrusted to a single Governmental Authority. The first Atomic Law in the Czech Republic is now prepared for approval by Parliament and will legally fulfill the rearrangement and establish an Office of Nuclear Safety and Radiation Protection.


OP65

THE LABORATORY-TYPE DATA INPUT AND PROCESSING SUBSYSTEM OF THE COUNTRY-WIDE ENVIRONMENTAL RADIATION MONITORING SYSTEM IN HUNGARY

B. Kanyar, N. Fulop, N. Glavatszkih, A. Nemeth

National Research Institute for Radiobiology and Radiohygiene, Budapest, Hungary

In Hungary the organisation of the nationwide environmental radiation monitoring is rather complex with several ministries, authorities and different types of laboratories involved. Therefore the Hungarian Atomic Energy Commission initiated some centralisation in the monitoring programme as a whole and data collection together with data analysis, dose assessments, decision support procedures etc. The National Research Institute for Radiobiology and Radiohygiene has had charged to direct the operative work and establish a central data bank, mainly for laboratory- type of data, in close cooperation with the different authorities and laboratories.

The information centre of the country-wide monitoring system has been equipped with a SUN SPARCserver-20 computer, INGRES data manager software and other main accessories. The data collection in the radiological laboratories is based on a local PC-network (Novell) with the running version of the INGRES and on-line connections to the centre by X.25 lines. As a first step of the development the user programs for data collections and some restricted processing written in INGRES were introduced for testing.

The data bank is to be operated both for normal and accidental situations with direct data transmission capabilities to the information center of the early warning system operated by the national organisations of the nuclear emergency. The extension of the number of laboratories is planned step-wise and the regular operation is to be started at the beginning of the next year with about 20 local stations.



OP66

AN OUTLOOK TO RADIATION PROTECTION DEVELOPMENT

R. Martincic, P. Strohal *

Jozef Stefan Institute, Jamova 39, Ljubljana, Slovenia
* Zagreb, Croatia

In view of the particular character of the radiation risks a system of radiation protection and safety has developed over many decades as the effects of ionizing radiation have been better and better understood.

Some events in the last decade had essential impact on radiation protection principles and doctrine. Among them are available data of some long term radio-epidemiological studies of populations exposed to radiation, several big radiation accidents and new data on measurable effects of chronic exposure resulting from natural radiation.

The evolution of radiation protection technology is expected to continue with improvements in instrumentation, modelling, assessment methods and quality control. Scientific knowledge constitutes an acceptable basis for a conservative system of protection. However, future scientific advances in biology might have a profound effect on many aspects of radiation protection. New practices are currently being developed or are expected to be introduced in near future.

All that indicates that, regardless of the achieved status of radiation protection, this is still a dynamic filed.

The assessment of the present status and possible future developments of radiation protection and safety are discussed in the paper in more detail.



Last update June 29, 1995